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The transition towards sustainable mobility encourages research into biofuels for use in internal combustion engines. For these alternative energy carriers, high-fidelity experimental data of flame speeds influenced by pressure, temperature, and air-fuel equivalence ratio under engine-relevant conditions are required to support the development of robust combustion models for spark-ignition engines. E.g., physicochemical-based approximation formulas adjusted to the fuel provide similar accuracy as high fidelity chemical kinetic model calculations at a fraction of the computational cost and can be easily adopted in engine simulation codes. In the present study, a workflow to enable predictive combustion engine modeling is applied first for a gasoline reference fuel and two biofuel blends recently proposed by Dahmen and Marquardt [Energy Fuels, 2017].

Oxygenated fuels such as polyoxymethylene dimethyl ethers (OME) offer a chance to significantly decrease emissions while switching to renewable fuels. However, compared to conventional diesel fuel, they have lower heating values and different evaporation behaviors which lead to differences in spray, mixture formation as well as ignition delay. In order to determine the mixture formation characteristics and the combustion behavior of neat OME3-5, optical investigations have been carried out in a high-pressure-chamber using shadowgraphy, mie-scatterlight and OH-radiation recordings. Liquid penetration length, gaseous penetration length, lift off length, spray cone angle and ignition delay have been determined and compared to those measured with diesel-fuel over a variety of pressures, temperatures, rail pressures and injection durations.

The demand for more efficient and clean engines have prompted the research and development of new engine technologies. Automotive engines expected to run with leaner mixtures and higher compression ratios. Lean burn is effective to increase fuel economy whilst reducing emissions but unreliable ignition of the lean mixtures by the conventional spark plug is one of the problems which causes concerns to the engine designers. Laser ignition is a promising technology and holds many benefits over the spark ignition because it can extend the ignitability of lean mixtures with flexibility of the ignition location and absence of electrode degradation for improved engine performance with lean burn. In this study, high-speed photography is used to investigate the flame kernel growth and propagation in an optical direct injection engine using laser ignition by an Nd:YAG laser.

Particle Number (PN) have already been a big issue for developing high efficiency internal combustion engines (ICEs). In this study, controlled spark-assisted stratified compression ignition (SSCI) with moderate end-gas auto-ignition was used for reducing PN in a high compression ratio gasoline direct injection (GDI) engine. Under wide open throttle (WOT) and Maximum Brake Torque timing (MBT) condition, high external cooled exhaust gas recirculation (EGR) was filled in the cylinder, while two-stage direct injection was used to form desired stoichiometric but stratified mixture. SSCI combustion mode exhibits two-stage heat release, where the first stage is associated with flame propagation induced by spark ignition and the second stage is the result of moderate end-gas auto-ignition without pressure oscillation at the middle or late stage of the combustion process.

A 1-Dimensional (1-D) model of fluid dynamic and chemistry kinetics following hot spot auto-ignition has been developed to simulate the process from auto-ignition to pressure wave propagation. The role of wall effect on the physical-chemical interaction process is numerically studied. A pressure wave is generated after hot spot auto-ignition and gradually damped as it propagates. The reflection of the wall forms a reflected pressure wave with twice the amplitude of the incident wave near the wall. The superposition of the reflected and forward pressure waves reinforces the intensity of the initial pressure wave. Wall effect is determined by the distance between the hot spot center and the cylinder wall. Hot spot auto-ignition near the wall easily initiates detonation under high-temperature and high-pressure conditions because pressure wave reflection couples with chemical reactions and propagates in the mixture with high reactivity.

2-Butanone (C4H8O) is a promising alternative fuel candidate as a pure as well as a blend component for substitution in standard gasoline fuels. It can be produced by the dehydrogenation of 2-butanol. To describe 2-butanone's basic combustion behaviour, it is important to investigate key physical properties such as the laminar burning velocity. The laminar burning velocity serves on the one hand side as a parameter to validate detailed chemical kinetic models. On the other hand, especially for engine simulations, various combustion models have been introduced, which rely on the laminar burning velocity as the physical quantity describing the progress of chemical reactions, diffusion, and heat conduction. Hence, well validated models for the prediction of laminar burning velocities are needed. New experimental laminar burning velocity data, acquired in a high pressure spherical combustion vessel, are presented for 1 atm and 5 bar at temperatures of 373 K and 423 K.

Maintaining low NOx emissions over the operating range of diesel engines continues to be a major issue. However, optical measurements of nitric oxide (NO) are lacking particularly in the core of diesel jets, i.e. in the region of premixed combustion close to the spray axis. This is basically caused by severe attenuation of both the laser light and fluorescent emission in laser-induced fluorescence (LIF) applications. Light extinction is reduced by keeping absorption path lengths relatively short in this work, by investigating diesel jets in a combustion vessel instead of an engine. Furthermore, the NO-detection threshold is improved by conducting 1-d line measurements instead of 2-d imaging. The NO-LIF data are corrected for light attenuation by combined LIF and spontaneous Raman scattering. The quantified maximum light attenuation is significantly lower than in comparable previous works, and its wavelength dependence is surprisingly weak.

With increasing interest in new biofuel candidates, 1-octanol and di-n-butylether (DNBE) were presented in recent studies. Although these molecular species are isomers, their properties are substantially different. In contrast to DNBE, 1-octanol is almost a gasoline-type fuel in terms of its auto-ignition quality. Thus, there are problems associated with engine start-up for neat 1-octanol. In order to find a suitable glow-plug position, mixture formation is studied in the cylinder under almost idle operating conditions in the present work. This is conducted by planar laser-induced fluorescence in a high-speed direct-injection optical diesel engine. The investigated C8-oxygenates are also significantly different in terms of their evaporation characteristics. Thus, in-cylinder mixture formation of these two species is compared in this work, allowing conclusions on combustion behavior and exhaust emissions.

Occurrence of sporadic super-knock is the main obstacle to the development of advanced gasoline engines. One of the possible inducements of super-knock, agglomerated soot particle induced pre-ignition, was studied for high boosted gasoline direct injection (GDI) engines. The correlation between soot emissions and super-knock frequency was investigated in a four-cylinder gasoline direct injection production engine. The test results indicate that higher in-cylinder soot emission correlate with more pre-ignition and super-knock cycles in a GDI production engine. To study the soot/carbon particles trigger super-knock, a single-cylinder research engine for super-knock study was developed. The carbon particles with different temperatures and sizes were introduced into the combustion chamber to trigger pre-ignition and super-knock.

Combustion behaviour and emissions characteristics of different blending ratios of diesel and gasoline fuels (Dieseline) were investigated in a light-duty 4-cylinder compression-ignition (CI) engine operating on partially premixed compression ignition (PPCI) mode. Experiments show that increasing volatility and reducing cetane number of fuels can help promote PPCI and consequently reduce particulate matter (PM) emissions while oxides of nitrogen (NOx) emissions reduction depends on the engine load. Three different blends, 0% (G0), 20% (G20) and 50% (G50) of gasoline mixed with diesel by volume, were studied and results were compared to the diesel-baseline with the same combustion phasing for all experiments. Engine speed was fixed at 1800rpm, while the engine load was varied from 1.38 to 7.85 bar BMEP with the exhaust gas recirculation (EGR) application.

n-butanol has been recognized as a promising alternative fuel for gasoline and may potentially overcome the drawbacks of methanol and ethanol, e.g. higher energy density. In this paper, the spray characteristics of gasoline and n-butanol have been investigated using a high pressure direct injection injector. High speed imaging and Phase Doppler Particle Analyzer (PDPA) techniques were used to study the spray penetration and the droplet atomization process. The tests were carried out in a high pressure constant volume vessel over a range of injection pressure from 60 to 150 bar and ambient pressure from 1 to 5 bar. The results show that gasoline has a longer penetration length than that of n-butanol in most test conditions due to the relatively small density and viscosity of gasoline; n-butanol has larger SMD due to its higher viscosity. The increase in ambient pressure leads to the reduction in SMD by 42% for gasoline and by 37% for n-butanol.

An experimental study of particulate matter (PM) emission was conducted on four cars from Chinese market. Three cars were powered by gasoline direct injection (GDI) engines and one car was powered by a port fuel injection (PFI) engine. Particulate mass, number and size distribution were measured based on a chassis dynamometer over new European driving cycle (NEDC). The particulate emission behaviors during cold start and hot start NEDCs were compared to understand how the running conditions influence particulate emission. Three kinds of gasoline with RON 91.9, 94.0 and 97.4 were tested to find the impact of RON on particulate emission. Because of time and facilities constraints, only one cold/hot start NEDC was conducted for every vehicle fueled with every fuel. The test results showed that more particles were emitted during cold start condition (first 200s in NEDC). Compared with cold start NEDC, the particulate mass and number of hot start NEDC decreased by a wide margin.

This paper studied the knock combustion process in gasoline HCCI engines. The complex chemical kinetics was implemented into the three-dimensional CFD code with LES (Large eddy simulation) to study the origin of the knock phenomena in HCCI combustion process. The model was validated using the experimental data from the cylinder pressure measurement. 3D-CFD with LES method gives detailed turbulence, species, temperature and pressure distribution during the gasoline HCCI combustion process. The simulation results indicate that HCCI engine knock originates from the random multipoint auto-ignition in the combustion chamber due to the slight inhomogeneity. It is induced by the significantly different heat release rate of high temperature oxidation (HTO) and low temperature oxidation (LTO) and their interactions.

Pilot injection (PI) during the negative-valve-overlap (NVO) period is one method to improve control of combustion in gasoline controlled auto-ignition engines. This is generally attributed to both chemical and thermal effects. However, there are little experimental data on active species formed by the combusting PI and their effect on main combustion in real engines. Thus, it is the objective of the current study to apply and assess optical in-cylinder diagnostics for these species. Firstly, the occurrence and nature of combustion during the NVO period is investigated by spectrally-resolved multi-species flame luminescence measurements. OH*, CH*, HCO*, CO-continuum chemiluminescence, and soot luminosity are recorded. Secondly, spectrally-, spatially-, and cycle-resolved laser-induced fluorescence measurements of formaldehyde are conducted. It is attempted to find a cycle-resolved measure of the chemical effect of PI.

Using EGR instead of throttle to control the load of a stoichiometric dual-fuel dieseline (diesel and gasoline) compression ignition (SDCI) engine with three-way catalyst (TWC) aftertreatment is considered a promising technology to address the challenges of fuel consumption and emissions in future internal combustion engines. High-speed imaging is used to record the flame signal in a single-cylinder optical engine with a PFI+DI dual injection system. The premixed blue flame is identified and separated using green and blue channels in RGB images. The effects of injection timing on SDCI combustion are studied. An earlier injection strategy is found to be ideal for soot reduction; however, the ignition-injection decoupling problem results in difficulties in combustion control. It is also found that a split injection strategy has advantages in soot reduction and thermal efficiency.

Little research has been done on spray characteristics of 2,5-dimethylfuran (DMF), since the breakthrough in its production method as an alternative fuel candidate. In this paper, the spray characteristics of pure fuels (DMF, Isooctane) and DMF-Isooctane blends under different ambient pressures (1 bar, 3 bar and 7 bar) and injection pressures (50 bar, 100 bar and 150 bar) were studied using Phase Doppler Particle Analyzer (PDPA) and high speed imaging. Droplet velocity, size distribution, spray angle and penetration of sprays were examined. Based on the results, DMF had larger SMD and penetration length than isooctane. The surface tension of fuel strongly influenced spray characteristics. Increasing the surface tension by 26 % resulted in 12 % increase in SMD. Higher ambient pressure increased the drag force, but SMD was not influenced by the increased drag force. However, the increased ambient pressure reduced the injection velocity and We number resulting in higher SMD.

Biodiesel is considered one of the most promising alternative fuels to petrol fuels. In this study, an attempt has been made to investigate and compare the effect of fuel injection pressure, injection timing, and exhaust gas recirculation (EGR) ratio on the particle size distributions and exhaust emissions of the diesel and biodiesel produced from waste cooking oil (WCO) used in a common rail direct injection (CRDI) diesel engine. The engine tests were conducted at two injection pressures (800 and 1600 bar), two injection timings (25 and 5 deg before top dead center (bTDC) and three EGR ratios (10%, 20% 30%) at a constant fuel injection energy per stroke and engine speed (1200 r/min). The results indicated that carbon monoxide (CO) and hydrocarbon (HC) emissions of biodiesel were slightly lower, but nitrogen oxide (NOx) emissions were slightly higher, than those of diesel fuel under most operating conditions.

Super knock which occurs in highly boosted spark ignition engines in low speed pre-ignition regime can lead to severe engine damage. However, super knock occurs occasionally, it is difficult to clearly identify the causes. The widely accepted assumption for the cause of this phenomenon is oil intrusion. Most of oils have been proved to have higher cetane number than n-heptane dose, indicating that the intruded oil is very liable to auto-ignition in a boosted engine. Although there have been reported the type of base oil and additive has significant effect on pre-ignition frequency, the oil induced super knock is still so far not supported by any direct evidence. This paper presents the effect of direct oil intrusion into cylinder on super knock. The experiment was carried out in a single cylinder engine. The diluted oil by gasoline with different ratio was directly injected into cylinder using a modified single-hole injector with 4MPa injection pressure.

High boost and direct injection hold the potential of enhanced power density and fuel consumption in the development of gasoline engines. However, super-knock with strong destructiveness was widely reported at low-speed and high-load operating regime in turbocharged GDI engines. The objective of this study is to clarify the characteristics of super-knock and to try to find some feasible solutions to suppress super-knock. To fast evaluate super-knock at low-speed and high-load regime, a rapid test procedure including three super-knock test sections of 5000 cycles with 3 idle operations, was proposed. The experimental data indicate that pre-ignition is not the sufficient condition for super-knock. Pre-ignition may lead to super-knock, heavy knock, slight knock, and non-knock. Compared with conventional knock, knock intensity of super-knock is much higher and the maximum amplitude of pressure rise at start of knock is more than one order of magnitude higher.

Homogeneous Charge Compression Ignition (HCCI) and Spark Ignition (SI) dual-mode operation provides a practical solution to apply HCCI combustion in gasoline engines. However, the different requirements of air-fuel ratio and EGR ratio between HCCI combustion and SI combustion results in enormous control challenges in HCCI/SI mode switch. In this paper, HCCI combustion was achieved in a four-cylinder gasoline direct injection engine without knock and misfire using close-loop control by knock index. Assisted Spark Stratified Compression Ignition (ASSCI) combustion was obtained stably at medium-high load. ASSCI combustion exhibits two-stage heat release with initial flame propagation and controlled auto-ignition. The knock index of ASSCI combustion is less than HCCI combustion due to the lower pressure rise rate.