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The societies around the world remain far from meeting the agreed primary goal outlined under the 2015 Paris Agreement on climate change: reducing greenhouse gas (GHG) emissions to keep global average temperature rise to well below 20°C by 2100 and making every effort to stay underneath of a 1.5°C elevation. Current emissions are rebounding from a brief decline during the economic downturn related to the Covid-19 pandemic. To get back on track to support the realization of the goal of the Paris Agreement, research suggests that GHG emissions should be roughly halved by 2030 on a trajectory to reach net zero by around mid-century.2 Although these are averaged global targets, every sector and country or market can and must contribute, especially higher-income and more developed countries bear the greater capacity to act. In 2020 direct tailpipe emissions from transport represented around 8 GtC02e, or nearly 15% of total emissions.

In this work, a transport and mixing model that calculates mixing in thermodynamic phase space was derived and validated. The mixing in thermodynamic multizone space is consistent to the one in the spatially resolved physical space. The model is developed using a turbulent channel flow as simplified domain. This physical domain of a direct numerical simulation (DNS) is divided into zones based on the quantitative value of transported scalars. Fluxes between the zones are introduced to describe mixing from the transport equation of the probability density function based on the mixing process in physical space. The mixing process of further scalars can then be carried out with these fluxes instead of solving additional transport equations. The relationship between the exchange flux in phase space and the concept of scalar dissipation are shown and validated by comparison to DNS results.

Pilot injection (PI) during the negative-valve-overlap (NVO) period is one method to improve control of combustion in gasoline controlled auto-ignition engines. This is generally attributed to both chemical and thermal effects. However, there are little experimental data on active species formed by the combusting PI and their effect on main combustion in real engines. Thus, it is the objective of the current study to apply and assess optical in-cylinder diagnostics for these species. Firstly, the occurrence and nature of combustion during the NVO period is investigated by spectrally-resolved multi-species flame luminescence measurements. OH*, CH*, HCO*, CO-continuum chemiluminescence, and soot luminosity are recorded. Secondly, spectrally-, spatially-, and cycle-resolved laser-induced fluorescence measurements of formaldehyde are conducted. It is attempted to find a cycle-resolved measure of the chemical effect of PI.

Both, the continuous strengthening of the exhaust emission legislation and the striving for a substantial reduction of carbon dioxide output in the traffic sector depict substantial requirements for the development of future diesel engines. These engines will comprise not only the mandatory diesel oxidation catalyst (DOC) and particulate filter DPF but a NOx aftertreatment system as well - at least for heavier vehicles. The oxidation catalysts as well as currently available NOx aftertreatment technologies, i.e., LNT and SCR, rely on sufficient exhaust gas temperatures to achieve a proper conversion. This is getting more and more critical due to the fact that today's and future measures for CO₂ reduction will result in further decrease of engine-out temperatures. Additionally this development has to be considered in the light of further engine electrification and hybridization scenarios.

The high-speed Dl-diesel engine has made a significant advance since the beginning of the 90's in the Western European passenger car market. Apart from the traditional advantage in fuel economy, further factors contributing to this success have been significantly improved performance and power density, as well as the permanent progress made in acoustics and comfort. In addition to the efforts to improve efficiency of automotive powertrains, the requirement for cleaner air increases through the continuous worldwide restriction of emissions by legislative regulations for diesel engines. Against the backdrop of global climate change, significant reduction of CO2 is observed. Hence, for the future, engine and vehicle concepts are needed, that, while maintaining the well-established attractive market attributes, compare more favorably with regard to fuel consumption.