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Hydrogen is widely considered a promising fuel for future transportation applications for both, internal combustion engines and fuel cells. Due to their advanced stage of development and immediate availability hydrogen combustion engines could act as a bridging technology towards a wide-spread hydrogen infrastructure. Although fuel cell vehicles are expected to surpass hydrogen combustion engine vehicles in terms of efficiency, the difference in efficiency might not be as significant as widely anticipated [1]. Hydrogen combustion engines have been shown capable of achieving efficiencies of up to 45 % [2]. One of the remaining challenges is the reduction of nitric oxide emissions while achieving peak engine efficiencies. This paper summarizes research work performed on a single-cylinder hydrogen direct injection engine at Argonne National Laboratory.

The 4th Workshop of the Engine Combustion Network (ECN) was held September 5-6, 2015 in Kyoto, Japan. This manuscript presents a summary of the progress in experiments and modeling among ECN contributors leading to a better understanding of soot formation under the ECN “Spray A” configuration and some parametric variants. Relevant published and unpublished work from prior ECN workshops is reviewed. Experiments measuring soot particle size and morphology, soot volume fraction (fv), and transient soot mass have been conducted at various international institutions providing target data for improvements to computational models. Multiple modeling contributions using both the Reynolds Averaged Navier-Stokes (RANS) Equations approach and the Large-Eddy Simulation (LES) approach have been submitted. Among these, various chemical mechanisms, soot models, and turbulence-chemistry interaction (TCI) methodologies have been considered.

As vehicle technology progresses to new levels of sophistication, so too, vehicle test methods must evolve. This is true for analytical testing in a laboratory and for on-road vehicle testing. Every year since 1993, the U.S. Department of Energy (DOE) and original equipment manufacturer (OEM) sponsors have organized a series of competitions featuring advanced hybrid electric vehicle (HEV) technology to develop and promote DOE goals in fuel savings and alternative fuel usage. The competition has evolved over many years and has included many alternative fuels feeding the prime mover (including hydrogen fuel cells). EcoCAR turned its focus to plug-in hybrid electric vehicles (PHEVs) and it was quickly realized that to keep using on-road testing methods to evaluate fuel and electricity consumption, a new method needed to be developed that would properly weight depleting operation with the sustaining operation, using the established Utility Factor (UF) method.

Given the importance of the fuel-injection process on the combustion and emissions performance of gasoline direct injected engines, there has been significant recent interest in understanding the fluid dynamics within the injector, particularly around the needle and through the nozzles. The pressure losses and transients that occur in the flow passages above the needle are also of interest. Simulations of these injectors typically use the nominal design geometry, which does not always match the production geometry. Computed tomography (CT) using x-ray and neutron sources can be used to obtain the real geometry from production injectors, but there are trade-offs in using these techniques. X-ray CT provides high resolution, but cannot penetrate through the thicker parts of the injector. Neutron CT has excellent penetrating power but lower resolution.

The performance of Gasoline Direct Injection (GDI) engines is governed by multiple physical processes such as the internal nozzle flow and the mixing of the liquid stream with the gaseous ambient environment. A detailed knowledge of these processes even for complex injectors is very important for improving the design and performance of combustion engines all the way to pollutant formation and emissions. However, many processes are still not completely understood, which is partly caused by their restricted experimental accessibility. Thus, high-fidelity simulations can be helpful to obtain further understanding of GDI injectors. In this work, advanced simulation and experimental methods are combined in order to study the spray characteristics of two different 3-hole GDI injectors.

Fuel cell vehicles are undergoing extensive research and development because of their potential for high efficiency and low emissions. Because fuel cell vehicles remain expensive and there is limited demand for hydrogen at present, very few fueling stations are being built. To try to accelerate the development of a hydrogen economy, some original equipment manufacturers in the automotive industry have been working on a hydrogen-fueled internal combustion engine (ICE) as an intermediate step. This paper compares the fuel economy potential of hydrogen powertrains to conventional gasoline vehicles. Several timeframes are considered: 2010, 2015, 2030, and 2045. To address the technology status uncertainty, a triangular distribution approach was implemented for each component technology. The fuel consumption and cost of five powertrain configurations will be discussed and compared with the conventional counterpart.

Fuel cell vehicles are the subject of extensive research and development because of their potential for high efficiency and low emissions. Because fuel cell vehicles remain expensive and the demand for hydrogen is therefore limited, very few fueling stations are being built. To try to accelerate the development of a hydrogen economy, some original equipment manufacturers (OEM) in the automotive industry have been working on a hydrogen-fueled internal combustion engine (ICE) as an intermediate step. Despite its lower cost, the hydrogen-fueled ICE offers, for a similar amount of onboard hydrogen, a lower driving range because of its lower efficiency. This paper compares the fuel economy potential of hydrogen-fueled vehicles to their conventional gasoline counterparts. To take uncertainties into account, the current and future status of both technologies were considered.

This paper analyzes fuel economy benefits of direct hydrogen and gasoline reformer fuel cell vehicles, with special focus on cold-start impacts on these fuel cell based vehicles. Comparing several existing influential studies reveals that the most probable estimates from these studies differ greatly on the implied benefits of both types of fuel cell vehicles at the tank-to-wheel level (vehicle-powertrain efficiency and/or specific power), leading to great uncertainties in estimating well-to-wheel fuel energy and/or greenhouse gas (GHG) emission reduction potentials. This paper first addresses methodological issues to influence the outcome of these analyses. With one exception, we find that these studies consistently ignore cold-start and warm-up issues, which play important roles in determining both energy penalties and start-up time of fuel cell vehicles. To better understand cold-start and warm-up behavior, this paper examines approaches and results based on two available U.S.

This study involves the battery requirements for a fuel cell-powered hybrid electric vehicle. The performances of the vehicle [a 3200-lb (1455-kg) sedan], the fuel cell, and the battery were evaluated in a vehicle simulation. Most of the attention was given to the design and performance of the battery, a lithium-ion, manganese spinel-graphite system of 75-kW power to be used with a 50-kW fuel cell. The total power performance of the system was excellent at the full operating temperatures of the fuel cell and battery. The battery cycling duty is very moderate, as regenerative braking for the Federal Urban Driving Schedule and the Highway Fuel Economy Test cycles can do all charging of the battery. Cold start-up at 20°C is straightforward, with full power available immediately.

Because of their high efficiency and low emissions, fuel-cell vehicles are undergoing extensive research and development. When considering the introduction of advanced vehicles, a complete well-to-wheel evaluation must be performed to determine the potential impact of a technology on carbon dioxide and Green House Gases (GHGs) emissions. Several modeling tools developed by Argonne National Laboratory (ANL) were used to evaluate the impact of advanced powertrain configurations. The Powertrain System Analysis Toolkit (PSAT) transient vehicle simulation software was used with a variety of fuel cell system models derived from the General Computational Toolkit (GCtool) for pump-to-wheel (PTW) analysis, and GREET (Green house gases, Regulated Emissions and Energy use in Transportation) was used for well-to-pump (WTP) analysis. This paper compares advanced propulsion technologies on a well-to-wheel energy basis by using current technology for conventional, hybrid and fuel cell technologies.

Because of their high efficiency and low emissions, fuel-cell vehicles are undergoing extensive research and development. As the entire powertrain system needs to be optimized, the requirements of each component to achieve FreedomCAR goals need to be determined. With the collaboration of FreedomCAR fuel cell, energy storage, and vehicle Technical Teams, Argonne National Laboratory (ANL) used several modeling tools to define the energy storage requirements for fuel cell vehicles. For example, the Powertrain System Analysis Toolkit (PSAT), which is a transient vehicle simulation software, was used with a transient fuel cell model derived from the General Computational Toolkit (GCtool). This paper describes the impact of degree of hybridization, control strategy, and energy storage technology on energy storage requirements for a fuel cell SUV vehicle platform.

This paper describes the integration of a Modal Energy and Emissions Model (MEEM) into a hybrid-electric vehicle simulation model, the PNGV System Analytic Toolkits (PSAT). PSAT is a forward-looking computer simulation model for advanced-technology vehicles. MEEM is a vehicle fuel-consumption and emissions model developed by one of the authors for internal-combustion-engine (ICE) -powered vehicles. MEEM engine simulation module uses a power-demand physical model based on a parameterized analytical representation of engine fuel and emissions production. One major advantage of MEEM is that it does not rely on steady-state engine maps, which are usually not available for most production vehicles; rather, it depends on a list of engine parameters that are calibrated based on regular vehicle dynamometer testing. The integrated PSAT-MEEM model can be used effectively to predict fuel consumption and emissions of various ICE-powered vehicles with both conventional and hybrid power trains.

A number of studies in the recent past have identified Laser Induced Incandescence (LII) as a versatile technique for measurement of soot concentration in flames. Recently, a number of researchers have focused their attention in adapting this technique to measure particulates in diesel exhausts. However, the agreement with established physical sampling techniques, such as the EPA recommended filter paper collection method, was found to be less than ideal. This paper reports our efforts to adapt this technique for diesel exhaust characterization. Many of the factors affecting LII signal were identified through computer modeling. Parameters that could not be determined through such a model were determined experimentally following a parametric study. Subsequently, LII measurements were performed in the exhaust of a modified lab burner, with conditions close to that of diesel engine exhausts.

Two limited-production hybrid electric vehicles (HEVs) - a 1988 Japanese model Toyota Prius and a 2000 Honda Insight - were tested at Argonne National Laboratory to collect data from vehicle component and systems operation. The test data are used to analyze operation and efficiency and to help validate computer simulation models. Both HEVs have FTP fuel economy greater than 45 miles per gallon and also have attributes very similar to those of conventional gasoline vehicles, even though each HEV has a unique powertrain configuration and operation control strategy. The designs and characteristics of these vehicles are of interest because they represent production technology with all the compromises for production included. This paper will explore both designs, their control strategies, and under what conditions high fuel economy was achieved.

The 2001 FutureTruck competition involved 15 universities from across North America that were invited to apply a wide range of advanced technologies to improve energy efficiency and reduce greenhouse gas impact while producing near-zero regulated exhaust emissions in a 2000 Chevrolet Suburban. The modified vehicles designated as FutureTrucks demonstrated improvements in greenhouse gas emissions, tailpipe emissions, and over-the-road fuel economy compared with the stock vehicle on which they were based. The technologies represented in the vehicles included ICE-engines and fuel cell hybrid electric vehicle propulsion systems, a range of conventional and alternative fuels, advanced exhaust emissions controls, and light weighting technologies.

Recent studies have indicated that substitutes for conventional petroleum resources will be needed to meet U.S. transportation energy demand in the first half of this century. One possible substitute is natural gas, which can be used as a transportation fuel directly in compressed natural gas or liquefied natural gas vehicles or as resource fuel for the production of hydrogen for fuel cell vehicles. This paper contains a preliminary assessment of the availability of U.S. natural gas resources to meet future U.S. transportation fuel demand. Several scenarios of natural gas demand, including transportation demand, in the United States to 2050 are developed. Natural gas resource estimates for the United States are discussed. Potential Canadian and Mexican exports to the United States are estimated. Two scenarios of potential imports from outside North America are also developed.

Several studies, conducted from 1997 to 2001, have employed vehicle and powertrain simulation models to estimate fuel economy gains for a variety of fuel-cell powertrains. Many of those studies have attempted to control for the comparability of performance between conventional and fuel-cell vehicles (FCVs), but different sets of performance goals and simulation models have been used. This paper reviews the estimates of fuel economy gain (in mpg) vs. varying measures of performance change for a set of those studies. We examine some of the potential causes for the variability of these estimates - fuel used, powertrain hybridization, vehicle raw energy requirements (load), and variations in analysts' assumptions/estimates - when substituting several types of fuel-cell powertrains. Our study includes development of a database and detailed examination of the relationships among powertrain and vehicle characteristics and fuel economy gain estimates for the selected studies.

The Department of Energyís Office of Advanced Automotive Technologies has been supporting the development of fuel-flexible fuel processors at Argonne National Laboratory. These fuel processors will enable fuel cell vehicles to operate on fuels available through the existing infrastructure. The constraints of on-board space and weight require that these fuel processors be compact and lightweight, while meeting the performance targets for efficiency and gas quality needed for the fuel cell. This paper discusses the performance of a prototype fuel processor that has been designed and fabricated to operate with liquid fuels, such as gasoline, ethanol, methanol, etc.

Onboard reforming of petroleum-based fuels, such as gasoline, may help ease the introduction of fuel cell vehicles to the marketplace. Although gasoline can be reformed, it is optimized to meet the demands of ICEs. This optimization includes blending to increase the octane number and addition of oxygenates and detergents to control emissions. The requirements for a fuel for onboard reforming to hydrogen are quite different than those for combustion. Factors such as octane number and flame speed are not important; however, factors such as hydrogen density, catalyst-fuel interactions, and possible catalyst poisoning become paramount. In order to identify what factors are important in a hydrocarbon fuel for reforming to hydrogen and what factors are detrimental, we have begun a program to test various components of gasoline and blends of components under autothermal reforming conditions. The results indicate that fuel composition can have a large effect on reforming behavior.

Süd-Chemie Inc. is producing and supplying an autothermal reforming (ATR) catalyst that was developed by Argonne National Laboratory (ANL) for reforming hydrocarbon fuels to generate H2 for automotive fuel cell systems. The catalyst is derived from solid oxide fuel cell technology, where a transition metal is supported on an oxide-ion-conducting substrate, such as ceria or zirconia, that is doped with an un-reducible oxide, such as gadolinium or samarium, to improve its oxide ion conductivity and to increase the number of surface oxygen ion vacancies. The catalyst has been shown to produce an H2-rich gas (reformate) from a wide variety of hydrocarbon fuels, including methane, natural gas, and commercial-grade gasolines and diesels with high selectivity. Platinum was the transition metal used in the first generation of the ANL catalyst.