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Diesel-fueled heavy-duty vehicles (HDVs) can be retrofitted with conversion kits to operate as dual-fuel vehicles in which partial diesel usage is offset by a gaseous fuel such as compressed natural gas (CNG). The main purpose of installing such a conversion kit is to reduce the operating cost of HDVs. Additionally, replacing diesel partially with a low-carbon fuel such as CNG can potentially lead to lower carbon dioxide (CO2) emissions in the tail-pipe. The main issue of CNG-diesel dual-fuel vehicles is the methane (CH4, the primary component of CNG) slip. CH4 is difficult to oxidize in the exhaust after-treatment (EAT) system and its slip may offset the advantage of lower CO2 emissions of natural gas combustion as CH4 is a strong greenhouse gas (GHG). The objective of this study is to compare the emissions of an HDV with a CNG conversion kit operating in diesel and dual-fuel mode during highway operation.