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With increased awareness and scrutiny of greenhouse gas (GHG) emissions, the heavy-duty truck industry is on the lookout for solutions that can maximize GHG savings, through either lowering fuel consumption and lowering methane slip. This paper focuses on whether it is possible to provide a differentiated Liquefied Natural Gas (LNG) that supports the further improvement of a High-Pressure Direct Injection (HPDI) Engine. Desired improvements from this LNG blend are the lowering or substitution of the pilot Diesel use of the current HPDI engine, the lowering of the raw exhaust gas methane concentration and any additional performance improvements. Sixty-five substances were identified that could potentially be blended into cryogenic methane thus creating a differentiated LNG fuel.