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In the field of vehicle aerodynamic simulation, Reynold Averaged Navier-Stokes (RANS) model is widely used due to its high efficiency. However, it has some limitations in capturing complex flow features and simulating large separated flows. In order to improve the computational accuracy within a suitable cost, the Field Inversion and Machine Learning (FIML) method, based on a data-driven approach, has received increasing attention in recent years. In this paper, the optimal coefficients of the Generalized k-ω (GEKO) model are firstly obtained by the discrete adjoint method of FIML, utilizing the results of wind tunnel experiments. Then, the mapping relationship between the flow field characteristics and the optimal coefficients is established by a neural network to augment the turbulence model.