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Lithium-ion battery has advantages of high energy density and cost effectiveness than other types of batteries. However due to the low mechanical stability, their performance is strongly influenced by environmental conditions. Especially, external pressure on a cell surface is a crucial factor because an appropriate force can improve battery cycle life, but excessive force may cause structural failure. In addition, battery pack is composed of various components so that uncertainties in dimension and material properties of each component can cause a wide variance in initial pressure. Therefore, it is important to optimize structural design of battery pack to ensure initial pressure in an effective range. In this paper, target stiffness of module structure was determined based on cell level cycle life test, then structural design has been optimized for weight reduction. Cell cycling tests were performed under different stiffness conditions and analyzed with regression model.