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The operating pressure is one of the critical issues in designing a gasoline-fueled PEM fuel cell system for transportation applications. Pressurized (3atm) and atmospheric pressure (1atm) fuel cell systems are being considered by various developers for automotive applications. Systems analyses have been performed for the two systems using GCtool, a computer simulation code developed at Argonne National Laboratory. The two systems were designed for comparable overall system efficiencies at a rated design power of 50 kW. The characteristics and performance of the different components of the two systems were compared at the design power and at part-load operating conditions. Transient analyses were performed to investigate the dynamic response of the two systems during cold startup. The pros and cons of the two systems regarding their performance, size, and preliminary cost estimates are presented.

A three phase catalytic mathematical model was developed for analysis and optimization of the volatile reactor assembly (VRA) used on International Space Station (ISS) Water Processor. The Langmuir-Hinshelwood Hougen-Watson (L-H) expression was used to describe the surface reaction rate. Small column experiments were used to determine the L-H rate parameters. The test components used in the experiments were acetic acid, acetone, ethanol, 1-propanol, 2-propanol and propionic acid. These compounds are the most prevalent ones found in the influent to the VRA reactor. The VRA model was able to predict performance of small column data and experimental data from the VRA flight experiment.