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In this study, a high-efficiency heavy-duty diesel engine platform was used to evaluate gasoline compression ignition (GCI) operation. The experiment was carried out using a single-cylinder engine (SCE) of a high compression ratio (22:1). Pump-grade gasoline fuel 87 research octane number (RON) was used throughout engine testing. Injection strategy was established including double and triple injection schemes to optimize both engine efficiency and emissions. Both low-temperature heat release (LTHR) and high-temperature heat release (HTHR) were seen from a two-stage combustion event resulting from the interaction of pilot and main injections. At low load conditions, besides fuel stratification level by pilot/main injection strategy, higher in-cylinder pressure can greatly improve the ignition of 1st stage combustion. As engine load increases, spray-wall interaction becomes more critical on engine efficiency and emissions performance.