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The effect of the chemical reactivity of diesel fuel on PM formation was investigated using a flow reactor and a shock tube. Reaction products from the flow-reactor pyrolysis of the three diesel fuels used for the engine tests in Part 1(1) (“Base”, “Improved” and Swedish “Class-1”) were analyzed by gas chromatography. At 850C, Swedish “Class-1” fuel was found to produce the most PM precursors such as benzene and toluene among the three fuels, even though it contains very low amounts of aromatics. The chemical analyses described in Part 1 revealed that “Class-1” contains a large amount of branched and cyclic structures in the saturated hydrocarbon portion of the fuel. These results suggest that the presence of such branched and ring structures can increase exhaust PM emissions.

This study models short circuits and blow-outs of spark channels. The short circuit model assumes that a spark channel is short-circuited between two arbitrary locations when the electric potential difference between the two locations exceeds the voltage which enables electrical insulation breakage in-between. The threshold voltage can be raised by increasing the distance between the two locations and decreasing the discharge current. Discharge current, in this model, represents the influence of both the spread and the number of electrically charged particles, i.e., electrons and positive ions, distributed near the two locations. Meanwhile, the blow-out model assumes that a strong flow diffuses electrons and positive ions in the spark channel, and consequently the discharge blows out.