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In the closed environment of an inhabited spacecraft, a critical aspect of the air revitalization system is the removal of the carbon dioxide (CO2) and water vapor produced by the crew. A number of different techniques can be used for CO2 removal, but current methods are either non-regenerative or require a relatively high power input for thermal regeneration. Two-bed CO2 adsorption systems that can remove CO2 from humid air and be regenerated using pressure-swing desorption offer mass, volume, and power advantages when compared with the other methods. Two classes of sorbent materials show particular promise for this application: Zeolite sorbents, similar to those in the International Space Station (ISS) CO2 removal assembly Functionalized carbon molecular sieves (FCMS), which adsorb CO2 independent of the humidity in the airstream Pressure-swing testing of these two different sorbents under both space station and space suit conditions are currently underway.