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This research focused on the light emission behavior of the OH radical (characteristic spectrum of 306.4 nm) that plays a key role in combustion reactions, in order to investigate the influence of the residual gas on autoignition. The test engine used was a 2-stroke, air-cooled engine fitted with an exhaust pressure control valve in the exhaust manifold. When a certain level of internal EGR is forcibly applied, the temperature of the unburned end gas is raised on account of heat transfer from the hot residual gas and also due to compression by piston motion. As a result, the unburned end gas becomes active and autoignition tends to occur.

Knocking is one phenomenon that can be cited as a factor impeding efforts to improve the efficiency of spark-ignition engines. With the aim of understanding knocking better, light emission spectroscopy was applied in this study to examine preflame reactions that can be observed prior to autoignition in the combustion reaction process of hydrocarbon fuels. Attention was focused on light emission behavior at wavelengths corresponding to those of formaldehyde (HCHO), Vaidya's hydrocarbon flame band (HCO) and the OH radical in a forced progression from normal combustion to a knocking state. Light emission behavior was measured simultaneously in the center and in the end zone of the combustion chamber when the engine was operated on two different test fuels. The test fuels used were n-heptane (0 RON) and a blended fuel (70 RON) consisting of n-heptane (0 RON) and iso-octane (100 RON).

With the aim of elucidating the mechanism causing abnormal combustion, a study was made of light emission and absorption characteristics at wavelengths corresponding to the spectra of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm), C2 (516.5 nm) radicals. Spectral properties were measured in the end-gas region of the cylinder for various types of fuel having different octane numbers. During combustion in an actual engine, the behavior of the CH and C2 radicals prior to the occurrence of abnormal combustion characterized by knock is indicative of behavior in the negative temperature coefficient (NTC) region. The experimental results revealed that the behavior of the OH, CH, C2 radicals differs between normal and abnormal combustion.

With the aim of elucidating the mechanism generating knock, an examination was made of the preflame reaction behavior of end gas in the combustion chamber in the transition from normal combustion to abnormal combustion characterized by the occurrence of knocking. Simultaneous measurements were made in the same cycle of the light absorption and emission behavior of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm) and C2 (516.5 nm) radicals in the end-gas region using spectroscopic methods. The absorbance behavior of a blue flame prior to autoignition is believed to be an important factor in the mechanism causing knock.

The investigation regarding the plasma jet ignition was explored by using a combustion vessel. The first purpose is to elucidate the issuing duration and the penetration of hydrogen plasma jet. A temporal change of local electron temperature was measured along the central axis of plasma jet. A small characteristic length of igniter seems favorable with regard to the plasma jet penetration and the generation of high temperature, as compared with the case of the igniter that has the excessive cavity volume. The second purpose is to elucidate relationship between the characteristic length and the combustion enhancement effect, when the excessive volume of cavity and the excessive supplied electrical energy were used. The influence of the characteristic length on the plasma jet penetration and the combustion enhancement differs with the supplied energy. The combustion enhancement seems to be caused by the plasma jet in case of excessive supplied energy.

The investigation regarding performance of plasma jet igniters was explored by using a constant volume vessel. This study focused on investigating the relationship between the jet effect, the hot gas jet issued from the igniter, and combustion enhancement. The hot gas penetration was visualized by the schlieren system with CCD camera and image intensifier. In the cases of small energies, 0.63 and 0.90 J, the combustion enhancement effect is similar to that of combustion jet igniter. In cases of supplied energies, 2.45 and 5.00 J, the jet effect influences on the combustion enhancement effect for small characteristic length of the igniter.

Using absorption spectroscopy, simultaneous measurements were made of the behavior of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm) and C2(516.5 nm) radicals in the end-gas region and center of the combustion chamber of a spark-ignition engine during preflame reactions with four types of fuel having different octane numbers. The results of this research show that the behavior of the OH, CH and C2 radicals in preflame reactions differed significantly in both the center and end-gas region of the combustion chamber depending on the octane number of the fuel and also between normal and knocking combustion conditions.

Emission intensity was measured at a wavelength of 395 2 nm (corresponding to the characteristic spectrum of the HCHO radical) and absorbance was measured at 306 4 nm (corresponding to that of the OH radical). The emission intensity and absorbance waveforms recorded during engine operation on n-heptane show behavior indicative of the passage and degeneracy of cool flame in the preflame reaction interval. As the combustion chamber wall temperature approached an overheated state in the transition from normal combustion to knocking operation different preflame reaction behavior was observed which is thought to correspond to the presence of a negative temperature coefficient region related to the ignition delay time.

We have investigated combustion characteristics of lean gasoline-air pre-mixture ignited by gas-oil injection using a high compression D.I. diesel engine. Gasoline was supplied as an uniform lean mixture by using carburetors, and gas-oil was directly injected into the cylinder. Two different types of combustion chamber were attempted. It was confirmed that the lean mixture of air-fuel ratio between 150 and 35 could be ignited and burned by this ignition method. An engine with the re-entrant type combustion chamber had an advantage for combustion and ignition. The brake mean effective pressure increased when relatively rich mixture was provided with a small amount of the gas-oil injection. As the gas-oil injection increased, HC concentration decreased, and NO and CO concentration increased. The exhaust gas emission of pollutants could be reduced when lean mixture was ignited by an optimum gas-oil injection.

The aim of this research was to investigate the mechanism causing autoignition and the effect of exhaust gas recirculation (EGR) on combustion by detecting the behavior of the OH radical and other excited molecules present in the flame in a spark ignition engine. The test equipment used was a 2-cycle engine equipped with a Schnürle scavenging system. Using emission spectroscopy, the behavior of the OH radical was measured at four locations in the end zone of the combustion chamber. The OH radical plays an important role in the elemental reactions of hydrocarbon fuels. When a certain level of EGR was applied according to the engine operating conditions, the unburned gas became active owing to heat transfer from residual gas near the measurement positions on the exhaust port side and the influence of excited species in the residual gas, and autoignition tended to occur.

The use of a higher compression ratio is desirable for improving the thermal efficiency and specific power of spark-ignition engines, but it gives rise to a problem of engine knock. In the present research, an investigation was made of the role of the preflame reaction region of a spark-ignition engine in the occurrence of autoignition. Emission spectroscopy was used to measure the behavior of formaldehyde (HCHO) in a cool flame. In addition, measure the behavior of the faint light attributed to the HCO radical in a blue flame with the concurrent measurement of the OH radical. The emission waveforms measurements obtained for HCHO when n-heptane (ORON) was used as the fuel, It is thought that these tendencies correspond to the passage and degeneracy of a cool flame. Further, the emission waveforms measured for the HCO radical when blended fuels (6ORON, 8ORON) were correspond to that of a blue flame.