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Current progress in the development of diesel engines substantially contributes to the reduction of NOx and Particulate Matter (PM) emissions but will not succeed to eliminate the application of Diesel Particulate Filters (DPFs) in the future. In the past we have introduced a Multi-Functional Reactor (MFR) prototype, suitable for the abatement of the gaseous and PM emissions of the Low Temperature Combustion (LTC) engine operation. In this work the performance of MFR prototypes under both conventional and advanced combustion engine operating conditions is presented. The effect of the MFR on the fuel penalty associated to the filter regeneration is assessed via simulation. Special focus is placed on presenting the performance assessment in combination with the existing differences in the morphology and reactivity of the soot particles between the different modes of diesel engine operation (conventional and advanced). The effect of aging on the MFR performance is also presented.

It is the objective of this work to characterize mixture formation in the sprays emanating from Multi-Layer (ML) nozzles under approximately engine-like conditions by quantitative, spatially, and temporally resolved fuel-air ratio and temperature measurements. ML nozzles are cluster nozzles which have more than one circle of orifices. They were introduced previously, in order to overcome the limitations of conventional nozzles. In particular, the ML design yields the potential of variable spray interaction, so that mixture formation could be controlled according to the operating condition. In general, it was also a primary aim of the cluster-nozzle concepts to combine the enhanced atomization and pre-mixing of small nozzle holes with the longer spray penetration lengths of large holes. The applied diagnostic, which is based on 1d spontaneous Raman scattering, yields the quantitative stoichiometric ratio and the temperature in the vapor phase.

In this study the fuel influence of several bio-fuel candidates on homogeneous engine combustion systems with direct injection is investigated. The results reveal Ethanol and 2-Butanol as the two most knock-resistant fuels. Hence these two fuels enable the highest efficiency improvements versus RON95 fuel ranging from 3.6% - 12.7% for Ethanol as a result of a compression ratio increase of 5 units. Tetrahydro-2-methylfuran has a worse knock resistance and a decreased thermal efficiency due to the required reduction in compression ratio by 1.5 units. The enleanment capability is similar among all fuels thus they pose no improvements for homogeneous lean burn combustion systems despite a significant reduction in NOX emissions for the alcohol fuels as a consequence of lower combustion temperatures.

It is a big challenge how to satisfy both the purification of exhaust gas and the decrease of fuel penalty, that is, carbon-dioxide emission. Regarding the Diesel Particulate Filter (DPF) applied in the diesel after-treatment system, it must be effective for lowering the fuel penalty to prolong the interval and reduce the frequency of the DPF regeneration operation. This can be achieved by a DPF that has high Particulate Matter (PM) mass limit and high PM oxidation performance that is enough to regenerate the DPF continuously during the normal running operation. In this study, the examination of the pore structure of the wall of a DPF that could expand the continuous regeneration region in the engine operation map was carried out. Several porous materials with a wide range of pore structure were prepared and coated with a Mixed Oxide Catalyst (MOC). The continuous regeneration performance was evaluated under realistic conditions in the exhaust of a diesel engine.

Direct catalytic soot oxidation is expected to become an important component of future diesel particulate emission control systems. The development of advanced Catalytic Diesel Particulate Filters (CDPFs relies on the interplay of chemistry and geometry in order to enhance soot-catalyst proximity. An extensive set of well-controlled experiments has been performed to provide direct catalytic soot oxidation rates in CDPFs employing small-scale side-stream sample exposure. The experiments are analyzed with a state-of-the-art diesel particulate filter simulator and a set of kinetic parameters are derived for direct catalytic soot oxidation by fuel-borne catalysts as well as by catalytic coatings. The influence of soot-catalyst proximity, on catalytic soot oxidation is found to be excellently described by the so-called Two-Layer model, developed previously by the authors.

The HSDI Diesel engine contributes substantially to the decrease of fleet fuel consumption thus to the reduction of CO2 emissions. This results in the rising market acceptance which is supported by desirable driving performance as well as greatly improved NVH behavior. In addition to the above mentioned requirements on driving performance, fuel economy and NVH behavior, continuously increasing demands on emissions performance have to be met. From today's view the Diesel particulate trap presents a safe technology to achieve the required reduction of the particle emission of more than 95%. However, according to today's knowledge a further, substantial NOx engine-out emission reduction for the Diesel engine is counteracts with the other goal of reduced fuel consumption. To comply with current and future emission standards, Diesel engines will require DeNOx technologies.

Novel catalytic coatings with a variety of methods based on conventional and novel synthesis routes are developed for Diesel Particulate Filters (DPFs). The developed catalytic composition exhibits significant direct soot oxidation as evaluated by reacting mixtures of diesel soot and catalyst powders in a thermogravimetric analysis apparatus (TGA). The catalyst composition was further deposited on oxide and non-oxide porous filter structures that were evaluated on an engine bench with respect to their filtration efficiency, pressure drop behavior and direct soot oxidation activity under realistic conditions. The effect of the catalyst amount on the filtration efficiency of non-oxide filters was also investigated. Evaluation of the indirect soot oxidation was conducted on non-oxide catalytic filters coated with precious metal.

A broad range of diesel, kerosene, and gasoline-like fuels has been tested in a single-cylinder diesel engine optimized for advanced combustion performance. These fuels were selected in order to better understand the effects of ignition quality, volatility, and molecular composition on engine-out emissions, performance, and noise levels. Low-level biofuel blends, both biodiesel (FAME) and ethanol, were included in the fuel set in order to test for short-term advantages or disadvantages. The diesel engine optimized in Part 1 of this study included cumulative engine hardware enhancements that are likely to be used to meet Euro 6 emissions limits and beyond, in part by operating under conditions of Homogeneous Charge Compression Ignition (HCCI), at least over some portions of the speed and load map.

Two single-cylinder diesel engines were optimised for advanced combustion performance by means of practical and cumulative hardware enhancements that are likely to be used to meet Euro 5 and 6 emissions limits and beyond. These enhancements included high fuel injection pressures, high EGR levels and charge cooling, increased swirl, and a fixed combustion phasing, providing low engine-out emissions of NOx and PM with engine efficiencies equivalent to today's diesel engines. These combustion conditions approach those of Homogeneous Charge Compression Ignition (HCCI), especially at the lower part-load operating points. Four fuels exhibiting a range of ignition quality, volatility, and aromatics contents were used to evaluate the performance of these hardware enhancements on engine-out emissions, performance, and noise levels.

Fuels derived from biomass will most likely contain oxygen due to the high amount of hydrogen needed to remove oxygen in the production process. Today, alcohol fuels (e. g. ethanol) are well understood for spark ignition engines. The Institute for Combustion Engines at RWTH Aachen University carried out a fuel investigation program to explore the potential of alcohol fuels as candidates for future compression ignition engines to reduce engine-out emissions while maintaining engine efficiency and an acceptable noise level. The soot formation and oxidation process when using alcohol fuels in diesel engines is not yet sufficiently understood. Depending on the chain length, alcohol fuels vary in cetane number and boiling temperature. Decanol possesses a diesel-like cetane number and a boiling point in the range of the diesel boiling curve. Thus, decanol was selected as an alcohol representative to investigate the influence of the oxygen content of an alcohol on the combustion performance.

Within the Cluster of Excellence “Tailor-Made Fuels from Biomass” at RWTH Aachen University, the Institute for Combustion Engines carried out an investigation program to explore the potential of future biofuel components in Diesel blends. In this paper, thermodynamic single cylinder engine results of today's and future biofuel components are presented with respect to their engine-out emissions and engine efficiency. The investigations were divided into two phases: In the first phase, investigations were performed with rapeseed oil methyl ester (B100) and an Ethanol-Gasoline blend (E85). In order to analyze the impact of different fuel blends, mixtures with 10 vol-% of B100 or E85 and 90 vol-% of standardized EN590 Diesel were investigated. Due to the low cetane number of E85, it cannot be used purely in a Diesel engine.

The DEXA Cluster consisted of three closely interlinked projects. In 2003 the DEXA Cluster concluded by demonstrating the successful development of critical technologies for Diesel exhaust particulate after-treatment, without adverse effects on NOx emissions and maintaining the fuel economy advantages of the Diesel engine well beyond the EURO IV (2000) emission standards horizon. In the present paper the most important results of the DEXA Cluster projects in the demonstration of advanced particulate control technologies, the development of a simulation toolkit for the design of diesel exhaust after-treatment systems and the development of novel particulate characterization methodologies, are presented. The motivation for the DEXA Cluster research was to increase the market competitiveness of diesel engine powertrains for passenger cars worldwide, and to accelerate the adoption of particulate control technology.

Diesel Particulate Filter (DPF) behavior depends strongly on the microstructural properties of the deposited soot aggregates. In the past the issue of the growth process of soot deposits in honeycomb ceramic filters has been addressed under non-reactive conditions and the influence of the filter operating conditions has been defined in terms of the dimensionless Peclet number. In the present work appropriate soot cake microstructural descriptors are studied under reactive conditions for different oxidation modes. To this end the effect of deposit microstructure on the soot oxidation kinetics is investigated. Different microstructural models for the reacting soot deposit are examined in a unified fashion and a generalized constitutive equation is obtained, describing several modes of microstructure evolution (shrinking layer, shrinking density, discrete columnar and continuous columnar).

A major challenge in the development of diesel filter systems is the selection of the appropriate filter medium in terms of its geometric configuration (cell density, wall thickness) and its physical properties (porosity, pore size). This selection aims to achieve minimization of the filter pressure drop as well as more efficient filter regeneration. The aim of the present work is to provide engineering criteria to support the design and selection of suitably sized wall-flow monolithic filters for diesel particulate control.

Environmental concern demands that emissions and fuel consumption of vehicles have to improve considerably in the next 10 years. New technologies for gasoline engines, downsizing with high boosting, direct injection and fully variable valve train systems, are being developed. For Diesel engines, improved components including piezobased injectors and particle filters are expected. In the drive train new starter-generator systems as well as automated manual transmissions are being developed. In parallel alternative fuels are investigated and the use of hybrid drives and fuel cells are developed. This paper reports the progress made in the recent years and gives a comparative assessment on the different technologies with a prediction of the introduction dates and volumes into the market.

The introduction of the new emission standards in 2002/04 for heavy-duty diesel engines requires a substantial reduction of the NOx emissions while the particulate emissions remain on a constant level. The application of cooled EGR appears to be the most common approach in order to achieve the required target, although other means such as advanced combustion systems and the application of emission control devices to reduce NOx emissions have to be taken into account as well. The purpose of this study is to investigate the potential of such alternative solutions in comparison with cooled EGR to meet the upcoming emission standards.

As demand for wall-flow Diesel particulate filters (DPF) increases, accurate predictions of DPF behavior, and in particular of the accumulated soot mass, under a wide range of operating conditions become important. This effort is currently hampered by a lack of a systematic knowledge of the accumulated particulate deposit microstructural properties. In this work, an experimental and theoretical study of the growth process of soot cakes in honeycomb ceramic filters is presented. Particular features of the present work are the application of first- principles measurement and simulation methodology for accurate determination of soot cake packing density and permeability, and their systematic dependence on the filter operating conditions represented by the Peclet number for mass transfer. The proposed measurement methodology has been also validated using various filters on different Diesel engines.

Diesel Particulate Filters (DPFs) need to be periodically regenerated in order to achieve efficient and safe vehicle operation. Under typical diesel exhaust conditions, this invariably requires the raising of the exhaust gas temperature by active means, up to the point that particulate (soot) oxidation can be self-sustained in the filter. In the present work the development path of an advanced catalytic filter technology is presented. Full scale optimized Catalytic Diesel Particulate Filters (CDPFs) are tested in the exhaust of a light-duty modern diesel engine in line with a Diesel Oxidation Catalyst (DOC). The management of the DOC-CDPF emission control system is facilitated by a virtual soot sensor in order to ensure energy-efficient operation of the emission control system.

The objective of this study is the design, construction and evaluation of a Selective Particle Size (SPS) sampler able to provide continuous delivery of diesel soot particles of specific size ranges. The design of the sampler combines principles of aerosol transport phenomena and separation technologies. Particles smaller than a given size are removed from the exhaust by diffusional deposition, while removal of particles above a given size is achieved by low pressure inertial impaction. The main application of the developed sampler is the exposure of biological samples such as cell and tissue cultures to selected sizes of diesel exhaust particles. By applying the SPS sampler to diesel exhaust it is demonstrated that it is possible to obtain two aerosol streams with widely separated particle size distributions (of nanometric dimensions), suitable for biological exposure studies.

In this paper a fast DPF screening procedure is proposed using small-scale filter samples of different technologies in a well-controlled environment but under realistic engine exhaust conditions. The DPF samples are evaluated in a specially built Multi-Reactor Assembly (MRA) with respect to their flow resistance, filtration efficiency, soot loading behavior, soot oxidation behavior, as well as their ash induced ageing behavior.