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Optimizing fuel injection spray is essential to comply with stringent future emission regulations for hybrid vehicles and internal combustion engine vehicles, and the spray characteristics and geometry must be robust for various engine operating conditions. This study presents experimental and numerical assessments of spray for lateral-mounted gasoline direct injection (GDI) sprays with different plume arrangements to analyze collapse characteristics, which can significantly deteriorate the geometry and characteristics of fuel sprays. Novel spray characterization methods are applied to analyze complex spray collapse behaviors using LED-based diffusive back-illuminated extinction imaging (DBIEI) and 3D computed tomographic (CT) image reconstruction. High-fidelity computational fluid dynamics (CFD) simulations are performed to analyze the detailed spray characteristics besides experimental characterization.