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Hydrogen-fueled homogeneous charge compression ignition (HCCI) engines have shown the ability to provide a cleaner and more efficient alternative to conventional fossil fuels. The use of hydrogen as a fuel has the potential to reduce greenhouse gas and promote sustainability. In this study, a modified single-cylinder Cooperative Fuel Research (CFR) engine was utilised to operate on hydrogen in a HCCI combustion mode under various compression ratio (CR) conditions. In the experiments, the amount of hydrogen injected was adjusted at each CR to maintain the crank angle at 50% mass fraction burned (CA50) combustion phasing at 3±1 crank angle degrees after top dead center or as lean as possible. The engine speed was fixed at 600 rpm, and the impact of different intake air temperatures was also investigated. The results indicated that as the compression ratio increases, the air-fuel ratio needs to be increased to maintain the desired CA50 value, i.e., the engine needs to operate leaner.