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Surface contamination, or soiling, of the exterior of road vehicles can be unsightly, can reduce visibility and customer satisfaction, and, with the increasing application of surface-mounted sensors, can degrade the performance of advanced driver-assistance systems. Experimental methods of evaluating surface contamination are increasingly used in the product development process, but the results are generally subjective. The use of computational methods for predicting contamination makes objective measures possible, but comparable data from experiment is an important validation requirement. This article describes the development of an objective measure of surface contamination arising during experiments. A series of controlled experiments using ultraviolet (UV) dye-doped water are conducted to develop a robust methodology. This process is then applied to a simplified contamination test.