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Residual stress prediction arising from manufacturing processes provides paramount information for the fatigue performance assessment of components subjected to cyclic loading. The determination of the material model to be applied in the numerical model should be taken carefully. This study focuses on the estimation of residual stresses generated after deep rolling of cast iron crankshafts. The researched literature on the field employs the available commercial material codes without closer consideration on their reverse loading capacities. To mitigate this gap, a single element model was used to compare potential material models with tensile-compression experiments. The best fit model was then applied to a previously developed crankshaft deep rolling numerical model. In order to confront the simulation outcomes, residual stresses were measured in two directions on real crankshaft specimens that passed through the same modeled deep rolling process.