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This work investigates the soot formation process in diesel jet flame using a detailed kinetic soot model implemented into the KIVA-3V multidimensional CFD code and 2D imaging by use of time-resolved laser induced incandescence (LII). The numerical model is based on the KIVA code which is modified to use CHEMKIN as the chemistry solver using Message Passing Interface (MPI). This allows for the chemical reactions to be simulated in parallel on multiple CPUs. The detailed soot model used is based on the method of moments, which begins with fuel pyrolysis, followed by the formation of polycyclic aromatic hydrocarbons, their growth and coagulation into spherical particles, and finally, surface growth and oxidation of the particles. The model can describe the spatial and temporal characteristics of soot formation processes such as soot precursors distributions, nucleation rate and surface reaction rate.

This paper confirms a structure for the soot formation process inside a burning diesel jet plume of oxygenated fuels. An explanation of how the soot formation process changes by the use of oxygenated fuel in comparison with that for using a conventional diesel fuel, and why oxygenated fuel drastically suppresses the soot formation has been derived from the chemical kinetic analysis. A detailed chemical kinetic mechanism, which is combined with various proposed chemical kinetic models including normal paraffinic hydrocarbon oxidation, oxygenated hydrocarbon oxidation, and poly-aromatic hydrocarbon (PAH) formation, was developed in present study. The calculated results are presented to elucidate the influence of fuel mixture composition and fuel structure, especially relating to oxygenated fuels, on PAH formation. The analysis also provides a new insight into the initial soot formation process in terms of the temperature range of PAH formation.

In SI engines with port injection system, the injected fuel spray adheres surely on the port wall and the inlet valve, consequently, the spray-wall interaction process leads to the generation of unburned hydrocarbons and uncontrollable mixture formation. This paper deals with the fuel mixture preparation process including basic research on characteristics of the wall-wetted fuel film on a flat wall inside a constant volume vessel. In the experiments, iso-octane mixed with biacetyl as a tracer dopant was injected through a pintle type injector against a flat glass wall under the ambient conditions of atmospheric pressure and room temperature. The thickness of the adhered fuel film on the wall was quantitatively measured by using laser induced fluorescence (LIF) technique, which provides 2-D distribution information with high special resolution as a function of the injection duration, the impingement distance from the injector to the wall, and the impingement angle against the wall.