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When performing catalyst modeling and parameter tuning it is desirable that the experimental data contain both transient and stationary points and can be generated over a short period of time. Here a method of creating such concentration transients for a full scale engine rig system is presented. The paper describes a valuable approach for changing the composition of engine exhaust gas going to a DOC (or potentially any other device) by conditioning the exhaust gas with an additional upstream DOC and/or SCR. By controlling the urea injection and the DOC bypass a wide range of exhaust compositions, not possible by only controlling the engine, could be achieved. This will improve the possibilities for parameter estimation for the modeling of the DOC.

Parameter tuning was performed against data from a full scale engine rig with a Diesel Oxidation Catalysts (DOC). Several different catalyst configurations were used with varying Pt loading, washcoat thickness and volume. To illustrate the interplay between kinetics and mass transport, engine operating points were chosen with a wide variation in variables (inlet conditions) and both transient and stationary operation was used. A catalyst model was developed where the catalyst washcoat was discretized as tanks in series both radially and axially. Three different model configurations were used for parameter tuning, evaluating three different approaches to modeling of internal transport resistance. It was concluded that for a catalyst model with internal transport resistance the best fit could be achieved if some parameters affecting the internal mass transport were tuned in addition to the kinetic parameters.

Achieving upcoming HD emissions legislation, Euro VI/EPA 10, is a challenge for all engine manufacturers. A likely solution to meet the NOx limit is to use a combination of EGR and SCR. Combining these two technologies poses new challenges and possibilities when it comes to optimization and calibration. Using a complete system approach, i.e., considering the engine and the aftertreatment system as a single unit, is important in order to achieve good performance. Optimizing the complete system is a tedious task; first there are a large number of variables which affect both emissions and fuel consumption (injection timing, EGR rate, urea dosing, injection pressure, pilot/post injections, for example). Secondly, the chemical reactions in the SCR catalyst are substantially slower than the dynamics of the diesel engine and the rest of the system, making the optimization problem time dependent.