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Cast aluminum alloys are used for cylinder heads in internal combustion engines to meet low weight and high strength (lightweight) design requirements. In the combustion chamber, the alloy experiences harsh operating conditions; i.e., temperature variation, constrained thermal expansion, chemical reaction, corrosion, oxidation, and chemical deposition. Under these conditions, thermomechanical fatigue (TMF) damage arises in the form of mechanical damage, environmental (oxidation) damage, and creep damage. In the present work, several important properties that influence the TMF life of the cylinder head have been identified through TMF and finite element analysis (FEA). The results show that improving the strength at high temperatures helps improve TMF life on the exhaust side of the head. On the other hand, improving strength and ductility extend TMF life at low temperature on the intake side.