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PEMFC (proton exchange membrane or polymer electrolyte membrane fuel cell) is a potential candidate as a future power source for automobile applications. Water and thermal management is important to PEMFC operation. Numerical models, which describe the transport and electrochemical phenomena occurring in PEMFCs, are important to the water and thermal management of fuel cells. 3D (three-dimensional) multi-scale CFD (computational fluid dynamics) models take into account the real geometry structure and thus are capable of predicting real operation/performance. In this study, a 3D multi-phase CFD model is employed to simulate a large-scale PEMFC (109.93 cm2) under various operating conditions. More specifically, the effects of operating pressure (1.0-4.0 atm) on fuel cell performance and internal water and thermal characteristics are studied in detail under two inlet humidities, 100% and 40%.

Proton exchange membrane fuel cell (PEMFC) provides a promising future low carbon automotive powertrain solution. The catalyst layer (CL) is its core component which directly influences the output performance. PEMFC performance can be greatly improved by the effective optimization of CL composition. This work demonstrates a deep optimization of CL composition for improving the PEMFC performance, including the platinum (Pt) loading, Pt percentage of carbon-supported Pt and ionomer to carbon ratio of the anode and the cathode,. The simulation results by a PEMFC three-dimensional (3D) computation fluid dynamics (CFD) model coupled with the CL agglomerate model is used to train the artificial neural network (ANN) which can efficiently predict the current density under different CL composition. Squared correlation coefficient (R-square) and mean percentage error in the training set and validation set are 0.9867, 0.2635% and 0.9543, 1.1275%, respectively.