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Reactivity controlled compression ignition (RCCI) is a potential combustion strategy to achieve high engine efficiency with ultra-low NOx and soot emissions. Fuel stratification can be used to control the heat release rate of RCCI combustion. But the in-cylinder combustion process of the RCCI under different fuel stratification degrees has not been well understood, especially at a higher engine load. In this paper, simultaneous measurement of natural flame luminosity and emission spectra was carried out on a light-duty optical RCCI engine under different fuel stratification degrees. The engine was run at 1200 revolutions per minute under a load about 7 bar indicated mean effective pressure (IMEP). In order to form fuel stratification degrees from low to high, the common-rail injection timing of n-heptane was changed from -180° CA after top dead center (ATDC) to -10° CA ATDC, while the iso-octane delivered in the intake stroke was fixed.