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Detailed chemistry and turbulence-chemistry interaction need to be properly taken into account for a realistic combustion simulation of IC engines where advanced combustion modes, multiple injections and stratified combustion involve a wide range of combustion regimes and require a proper description of several phenomena such as auto-ignition, flame stabilization, diffusive combustion and lean premixed flame propagation. To this end, different approaches are applied and the most used ones rely on the well-stirred reactor or flamelet assumption. However, well-mixed models do not describe correctly flame structure, while unsteady flamelet models cannot easily predict premixed flame propagation and triple flames. A possible alternative for them is represented by transported probability density functions (PDF) methods, which have been applied widely and effectively for modeling turbulent reacting flows under a wide range of combustion regimes.

A transparent HSDI CI engine was used together with a high speed camera to analyze the liquid phase spray geometry of the fuel types: Swedish environmental class 1 Diesel fuel (MK1), Soy Methyl Ester (B100), n-Heptane (PRF0) and a gas-to-liquid derivate (GTL) with a distillation range similar to B100. The study of the transient liquid-phase spray propagation was performed at gas temperatures and pressures typical for start of injection conditions of a conventional HSDI CI engine. Inert gas was supplied to the transparent engine in order to avoid self-ignition at these cylinder gas conditions. Observed differences in liquid phase spray geometry were correlated to relevant fuel properties. An empirical relation was derived for predicting liquid spray cone angle and length prior to ignition.

HCCI mode has shown its potential to improve emissions and efficiency in internal combustion engines. In addition, it has open the possibility to use a wider range of fuels than in SI and CI engines. However, the engine running zone is still one of the main challenges that HCCI has to face. We have investigated this zone in the case of ethyl acetate using CFD simulations with a simplified combustion mechanism. This paper describes how ethyl acetate influences the running zone of HCCI engines compared to iso-octane. Biochemical conversion of fermentable biomass can produce large quantities of esters by the reaction of ethanol with volatile organic acids. Among them, ethyl acetate has a low vaporization temperature and a high auto-ignition temperature. Preliminary experiments on SI engines have shown that it ignites more slowly than gasoline even if their physical properties are similar.

Multi-dimensional models represent today consolidated tools to simulate the combustion process in HCCI and diesel engines. Various approaches are available for this purpose, it is however widely accepted that detailed chemistry represents a fundamental prerequisite to obtain satisfactory results when the engine runs with complex injection strategies or advanced combustion modes. Yet, integrating such mechanisms generally results in prohibitive computational cost. This paper presents a comprehensive methodology for fast and efficient simulations of combustion in internal combustion engines using detailed chemistry. For this purpose, techniques to tabulate the species reaction rates and to reduce the chemical mechanisms on the fly have been coupled.

Some fuels with the same research octane number (RON) have different HCCI engine performance. Therefore RON alone cannot be used for determining auto-ignition in HCCI combustion. The current research focuses on creating an HCCI fuel index suitable for comparing different fuels for HCCI operation. More thorough studies are needed to map the fuel effects. One way to characterize a fuel is by using the Auto-Ignition Temperature (AIT). The AIT and the amount of Low Temperature Heat Release (LTHR) together describe the auto-ignition properties of the fuel. Both can be extracted from the pressure trace. The assumption is that the pressure and temperature are known at inlet valve closing (IVC) and that the mass in the cylinder does not change after IVC. The purpose of this study was to map the AIT of different Primary Reference Fuels (PRF) for HCCI combustion at different cylinder pressures.

An index to relate fuel properties to HCCI auto-ignition would be valuable to predict the performance of fuels in HCCI engines from their properties and composition. The indices for SI engines, the Research Octane Number (RON) and Motor Octane Number (MON) are known to be insufficient to explain the behavior of oxygenated fuels in an HCCI engine. One way to characterize a fuel is to use the Auto-Ignition Temperature (AIT). The AIT can be extracted from the pressure trace. Another potentially interesting parameter is the amount of Low Temperature Heat Release (LTHR) that is closely connected to the ignition properties of the fuel. A systematic study of fuels consisting of gasoline surrogate components of n-heptane, iso-octane, toluene, and ethanol was made. 21 fuels were prepared with RON values ranging from 67 to 97.

While the optimization of the internal combustion engine (ICE) remains a very important topic, alternative fuels are also expected to play a significant role in the reduction of CO2 emissions. High energy densities and handling ease are their main advantages amongst other energy carriers. Ammonia (NH3) additionally contains no carbon and has a worldwide existing transport and storage infrastructure. It could be produced directly from renewable electricity, water and air, and is thus currently considered as a smart energy carrier and combustion fuel. However, ammonia presents a low combustion intensity and the risk of elevated nitrogen-based emissions, thus rendering in-depth investigation of its suitability as an ICE fuel necessary. In the present study, a recent single-cylinder spark-ignition engine is fueled with gaseous ammonia/hydrogen/air mixtures at various hydrogen fractions, equivalence ratios and intake pressures.

The transportation sector adds to the greenhouse gas emissions worldwide. One way to decrease this impact from transportation is by using renewable fuels. Ethanol is a readily available blend component which can be produced from bio blend­stock, currently used blended with gasoline from low to high concentrations. This study focuses on a high octane (RON=97) gasoline blended with 0, 20, and 50, volume % of ethanol, respectively. The high ethanol blended gasoline was used in a light duty engine originally designed for diesel combustion. Due to the high octane rating and high ignition resistance of the fuel it required high intake temperatures of 443 K and higher to achieve stable combustion in in homogeneously charged compression ignition (HCCI) combustion operation at low load. To enable combustion with lower intake temperatures more commonly used in commercial vehicles, ozone was injected with the intake air as an ignition improver.

An HSDI Diesel engine was fuelled with standard Swedish environmental class 1 Diesel fuel (MK1), Soy methyl ester (B100) and n-heptane (PRF0) to study the effects of both operating conditions and fuel properties on engine performance, resulting emissions and spray characteristics. All experiments were based on single injection diesel combustion. A load sweep was carried out between 2 and 10 bar IMEPg. For B100, a loss in combustion efficiency as well as ITE was observed at low load conditions. Observed differences in exhaust emissions were related to differences in mixing properties and spray characteristics. For B100, the emission results differed strongest at low load conditions but converged to MK1-like results with increasing load and increasing intake pressures. For these cases, spray geometry calculations indicated a longer spray tip penetration length. For low-density fuels (PRF0) the spray spreading angle was higher.

Experiments are performed in optical engines in order to understand the combustion process in standard engines. In spite of this, little work has been done to verify that the results from optical engines are representative for a standard engine. The wall heat losses in optical engines are lower than in all-metal engines due to the lower heat conductivity of optical parts and a less efficient cooling system. Furthermore, optical engines often have larger crevice volumes due to a lower position of the piston rings. The present investigation studies how these differences affect the heat release and emissions in optical HSDI diesel engines. Five different engine configurations are studied: an optical engine of Bowditch design with two different squish heights, the same engine fitted with a metal piston, the same engine with all quartz parts replaced with metal components and, finally, a standard diesel engine. It is found that the use of optical parts affect the combustion process.

The Diesel Particulate Filter (DPF) is the most effective way to reduce particulate matter emissions from diesel vehicles and is fitted on every passenger car since the EURO5 emission standard. Unfortunately, this essential after-treatment device can be damaged over time or could be defective from the manufacturing, negatively impacting its filtration efficiency. It is also sometimes illegally removed. Today in Europe, the presence and effectiveness of the DPF cannot be determined at the Periodic Technical Inspection (PTI), during which an opacity measurement of the exhaust gases is performed during a free acceleration test. Therefore, this work presents the results of the feasibility study of a new test procedure using devices measuring a particulate matter concentration (PN). The test consists of a PN measurement at low idle, which shows good correlation with NEDC PN emissions.

Homogeneous charge compression ignition (HCCI) is a promising concept that can be used to reduce NOx and soot emissions in combustion engines, keeping efficiency as high as for diesel engines. To be able to accurately control the combustion behavior, more information is needed about the auto-ignition of fuels. Many fuels, especially those containing n-paraffins, exhibit pre-reactions before the main heat release event, originating from reactions that are terminated when the temperature in the cylinder reaches a certain temperature level. These pre-reactions are called low temperature heat release (LTHR), and are known to be affected by engine speed. This paper goes through engine speed effects on auto-ignition temperatures and LTHR for primary reference fuels. Earlier studies show effects on both quantity and timing of the low temperature heat release when engine speed is varied.

As an alternative to second generation ethanol, valeric esters can be produced from lignocellulose through levulinic acid. While some data on these fuels are available, only few experiments have been performed to analyze their combustion characteristics under engine conditions. Using a traditional spark ignition engine converted to mono-cylinder operation, we have investigated the engine performances and emissions of methyl and ethyl valerates. This paper compares the experimental results for pure valeric esters and for blends of 20% of esters in PRF95, with PRF95 as the reference fuel. The esters propagate faster than PRF95 which requires a slight change of ignition timing to optimise the work output. However, both the performances and the emissions are not significantly changed compared to the reference. Accordingly, methyl and ethyl valerate represent very good alternatives as biofuels for SI engines.

HCCI combustion can be enabled by many types of liquid and gaseous fuels. When considering what fuels will be most suitable, the emissions also have to be taken into account. This study focuses on the emissions formation originating from different fuel components. A systematic study of over 40 different gasoline surrogate fuels was made. All fuels were studied in a CFR engine running in HCCI operation. Many of the fuels were blended to achieve similar RON's and MON's as gasoline fuels, and the components (n-heptane, iso-octane, toluene, and ethanol) were chosen to represent the most important in gasoline; nparaffins, iso-paraffins, aromatics and oxygenates. The inlet air temperature was varied from 50°C to 150°C to study the effects on the emissions. The compression ratio was adjusted for each operating point to achieve combustion 3 degrees after TDC. The engine was run at an engine speed of 600 rpm, with ambient intake air pressure and with an equivalence ratio of 0.33.

This study examines fuel auto-ignitability and shows a method for determining fuel performance for HCCI combustion by doing engine experiments. Previous methods proposed for characterizing HCCI fuel performance were assessed in this study and found not able to predict required compression ratio for HCCI auto-ignition (CRAI) at a set combustion phasing. The previous indices that were studied were the Octane Index (OI), developed by Kalghatgi, and the HCCI Index, developed by Shibata and Urushihara. Fuels with the same OI or HCCI Index were seen to correspond to a wide range of compression ratios in these experiments, so a new way to describe HCCI fuel performance was sought. The Lund-Chevron HCCI Number was developed, using fuel testing in a CFR engine just as for the indices for spark ignition (research octane number and motor octane number, RON and MON) and compression ignition (cetane number, CN).

A new multi-zone model for the simulation of HCCI engine is here presented. The model includes laminar and turbulent diffusion and conduction exchange between the zones and the last improvements on the numerical aspects. Furthermore, a new strategy for the zone discretization is presented, which allows a better description of the near-wall zones. The aim of the work is to provide a fast and reliable model for carrying out chemical analysis with detailed kinetic schemes. A preliminary sensitivity analysis allows to verify that 10 zones are a convenient number for a good compromise between the computational effort and the description accuracy. The multi-zone predictions are then compared with the CFD ones to find the effective turbulence parameters, with the aim to describe the near-wall phenomena, both in a reactive and non-reactive cases.

Experiments on a modern DI Diesel engine were carried out: The engine was fuelled with standard Diesel fuel, RME and a mixture of 85% standard Diesel fuel, 5% RME and 10% higher alcohols under low load conditions (4 bar IMEP). During these experiments, different external EGR levels were applied while the injection timing was chosen in a way to keep the location of 50% heat release constant. Emission analysis results were in accordance with widely known correlations: Increasing EGR rates lowered NOx emissions. This is explained by a decrease of global air-fuel ratio entailing longer ignition delay. Local gas-fuel ratio increases during ignition delay and local combustion temperature is lowered. Exhaust gas analysis indicated further a strong increase of CO, PM and unburned HC emissions at high EGR levels. This resulted in lower combustion efficiency. PM emissions however, decreased above 50% EGR which was also in accordance with previously reported results.

The current research focus on fuel effects on low temperature reactions (LTR) in Homogeneous Charge Compression Ignition (HCCI) and Partially Premixed Combustion (PPC). LTR result in a first stage of heat release with decreasing reaction rate at increasing temperature. This makes LTR important for the onset of the main combustion. However, auto-ignition is also affected by other parameters and all fuel does not exhibit LTR. Moreover, the LTR does not only depend on fuel type but also on engine conditions. This research aims to understand how fuel composition affects LTR in each type of combustion mode and to determine the relative importance of chemical and physical fuel properties for PPC. For HCCI the chemical properties are expected to dominate over physical properties, since vaporization and mixing are completed far before start of combustion.

Ammonia is now recognized as a very serious asset in the context of the hydrogen energy economy, thanks to its non-carbon nature, competitive energy density and very mature production, storage and transport processes. If produced from renewable sources, its use as a direct combustion fuel could participate to the flexibility in the power sector as well as help mitigating fossil fuel use in certain sectors, such as long-haul shipping. However, ammonia presents unfavorable combustion properties, requiring further investigation of its combustion characteristics in practical systems. In the present study, a modern single-cylinder spark-ignition engine is fueled with gaseous ammonia/air mixtures at various equivalence ratios and intake pressures. The results are compared with methane/air and previous ammonia/hydrogen/air measurements, where hydrogen is used as combustion promoter. In-cylinder pressure and exhaust concentrations of selected species are measured and analyzed.

Ammonia and hydrogen can be produced from water, air and excess renewable electricity (Power-to-fuel) and are therefore a promising alternative in the transition from fossil fuel energy to cleaner energy sources. An Homogeneous-Charge Compression-Ignition (HCCI) engine is therefore being studied to use both fuels under a variable blending ratio for Combined Heat and Power (CHP) production. Due to the high auto-ignition resistance of ammonia, hydrogen is required to promote and stabilize the HCCI combustion. Therefore the research objective is to investigate the HCCI combustion of varying hydrogen-ammonia blending ratios in a 16:1 compression ratio engine. A specific focus is put on maximizing the ammonia proportion as well as minimizing the NOx emissions that could arise from the nitrogen contained in the ammonia. A single-cylinder, constant speed, HCCI engine has been used with an intake pressure varied from 1 to 1.5 bar and with intake temperatures ranging from 428 to 473 K.