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Schlieren and shadowgraph imaging have been used for many years to identify refractive index gradients in various applications. For evaporating fuel sprays, these techniques can differentiate the boundary between spray regions and background ambient gases. Valuable information such as the penetration rate, spreading angle, spray structure, and spray pattern can be obtained using schlieren diagnostics. In this study, we present details of a z-type schlieren system setup and its application to port-fuel-injection gasoline sprays. The schlieren high-speed movies were used to obtain time histories of the spray penetration and spreading angle. Later, these global parameters were compared to specifications provided by the injector manufacturer. Also, diagnostic parameters such as the proportion of light cut-off at the focal point and the orientation of knife-edge (schlieren-stop) used to achieve the cut-off were examined.

The enhancement of vortex development, fuel-air mixing and heat release in diesel spray flame by inversed-delta injection rate shaping, having been predicted via LES simulation with detailed chemical kinetics, is experimentally confirmed for the first time. Newly developed 3-injector TAIZAC (TAndem Injector Zapping ACtivation) injector realizing aggressive inversed-delta injection rate shaping was used for single-shot combustion experiments in a constant volume combustion vessel. Simultaneous high-speed (120,000fps) and high-resolution (1,280 x 704 pixels) laser schlieren and UV OH* chemiluminescence imaging combined with subsequent Flame Imaging Velocimetry (FIV) analysis was employed to elucidate the correlation between vortex development and enhanced heat release.

Shadowgraph/schlieren imaging techniques have often been used for flow visualization of reacting and non-reacting systems. In this paper we show that high-speed shadowgraph visualization in a high-pressure chamber can also be used to identify cool-flame and high-temperature combustion regions of diesel sprays, thereby providing insight into the time sequence of diesel ignition and combustion. When coupled to simultaneous high-speed Mie-scatter imaging, chemiluminescence imaging, pressure measurement, and spatially-integrated jet luminosity measurements by photodiode, the shadowgraph visualization provides further information about spray penetration after vaporization, spatial location of ignition and high-temperature combustion, and inactive combustion regions where problematic unburned hydrocarbons exist. Examples of the joint application of high-speed diagnostics include transient non-reacting and reacting injections, as well as multiple injections.

For better understanding of soot formation and oxidation processes applicable to diesel engines, the size, morphology, and nanostructure of soot particles directly sampled in a diesel spray flame generated in a constant-volume combustion chamber have been investigated using Transmission Electron Microscopy (TEM). For this soot diagnostics, the effects of the sampling processes, TEM observation methodology and image processing methods on the uncertainty in the results have not been extensively discussed, mainly due to the complexity of the analysis.

Two-stage fuel direct injection (DI) has the potential to expand the operating region and control the auto-ignition timing in a Diesel fuelled homogeneous charge compression ignition (HCCI) engine. In this work, to investigate the dual-injection HCCI combustion, a stochastic reactor model, based on a probability density function (PDF) approach, is utilized. A new wall-impingement sub-model is incorporated into the stochastic spray model for direct injection. The model is then validated against measurements for combustion parameters and emissions carried out on a four stroke HCCI engine. The initial results of our numerical simulation reveal that the two-stage injection is capable of triggering the charge ignition on account of locally rich fuel parcels under certain operating conditions, and consequently extending the HCCI operating range.

Implementing triple injection strategies in partially premixed charge-based gasoline compression ignition (GCI) engines has shown to achieve improved engine efficiency and reduced NOx and smoke emissions in many previous studies. While the impact of the triple injections on engine performance and engine-out emissions are well known, their role in controlling the mixture homogeneity and charge premixedness is currently poorly understood. The present study shows correspondence between the triple injection strategies and mixture homogeneity/premixedness through the experimental tests of second/third injection proportion and their timing variations with an aim to explain the observed GCI engine performance and emission trends. The experiments were conducted in a single cylinder, small-bore common-rail diesel engine fuelled with a commercial gasoline fuel of 95 research octane number (RON) and running at 2000 rpm and 830 kPa indicated mean effective pressure conditions.

For a better understanding of soot formation and oxidation processes in conventional diesel and biodiesel spray flames, the morphology, microstructure and sizes of soot particles directly sampled in spray flames fuelled with US#2 diesel and soy-methyl ester were investigated using transmission electron microscopy (TEM). The soot samples were taken at 50mm from the injector nozzle, which corresponds to the peak soot location in the spray flames. The spray flames were generated in a constant-volume combustion chamber under a diesel-like high pressure and high temperature condition (6.7MPa, 1000K). Direct sampling permits a more direct assessment of soot as it is formed and oxidized in the flame, as opposed to exhaust PM measurements. Density of sampled soot particles, diameter of primary particles, size (gyration radius) and compactness (fractal dimension) of soot aggregates were analyzed and compared. No analysis of the soot micro-structure was made.

The NO reduction in an ammonia SCR converter has been simulated by a 1D+1D model for a single representative channel to parametrically study the characteristics of the system under typical operating conditions. An appropriate model has been selected interpreting the chemical behavior of the system and the parameters are calibrated based on a comprehensive set of experiments with an Fe-Zeolite washcoated monolith for different feed concentrations, temperatures and flow rates. Physical and chemical properties are determined as well as kinetics and rate parameters and the model has been verified by experimental data at different operating conditions. Three different mechanisms for the surface kinetics to model NO reduction have been assessed and the results have been compared in the cases of steady DeNO performance and transient response of the system. Ammonia inhibition is considered in the model since it has a major effect specifically under transient operating conditions.

Diesel low-temperature combustion strategies often rely on early injection timing to allow sufficient fuel-ambient mixing to avoid NOx and soot-forming combustion. However, these early injection timings permit the spray to penetrate into a low ambient temperature and density environment where vaporization is poor and liquid impingement upon the cylinder liner and piston bowl are more likely to occur. The objective of this study is to measure the transient liquid and vapor penetration at early-injection conditions. High-speed Mie-scatter and shadowgraph imaging are employed in an optically accessible chamber with a free path of 100 mm prior to wall impingement and using a single-spray injector. The ambient temperature and density within the chamber are well-controlled (uniform) and selected to simulate in-cylinder conditions when injection occurs at -40 crank-angle degrees (CAD) or fewer before top-dead center (TDC).

The effects of charge dilution on low-temperature diesel combustion and emissions were investigated in a small-bore single-cylinder diesel engine over a wide range of injection timing. The fresh air was diluted with additional N2 and CO2, simulating 0 to 65% exhaust gas recirculation in an engine. Diluting the intake charge lowers the flame temperature T due to the reactant being replaced by inert gases with increased heat capacity. In addition, charge dilution is anticipated to influence the local charge equivalence ratio ϕ prior to ignition due to the lower O2 concentration and longer ignition delay periods. By influencing both ϕ and T, charge dilution impacts the path representing the progress of the combustion process in the ϕ-T plane, and offers the potential of avoiding both soot and NOx formation.

Particle image velocimetry measurements of the in-cylinder flow in an optically accessible single-cylinder research engine were taken to better understand the effects of intake pressure variations on the flow field. At a speed of 1500 rpm, the engine was run at six different intake pressure loads from 0.4 to 0.95 bar under motored operation. The average velocity fields show that the tumble center position is located closer to the piston and velocity magnitudes decrease with increasing pressure load. A closer investigation of the intake flow near the valves reveals sharp temporal gradients and differences in maximum and minimum velocity with varying intake pressure load which are attributed to intake pressure oscillations. Despite measures to eliminate acoustic oscillations in the intake system, high-frequency pressure oscillations are shown to be caused by the backflow of air from the exhaust to the intake pipe when the valves open, exciting acoustic modes in the fluid volume.

Engine-out CO emission and fuel conversion efficiency were measured in a highly-dilute, low-temperature diesel combustion regime over a swirl ratio range of 1.44-7.12 and a wide range of injection timing. At fixed injection timing, an optimal swirl ratio for minimum CO emission and fuel consumption was found. At fixed swirl ratio, CO emission and fuel consumption generally decreased as injection timing was advanced. Moreover, a sudden decrease in CO emission was observed at early injection timings. Multi-dimensional numerical simulations, pressure-based measurements of ignition delay and apparent heat release, estimates of peak flame temperature, imaging of natural combustion luminosity and spray/wall interactions, and Laser Doppler Velocimeter (LDV) measurements of in-cylinder turbulence levels are employed to clarify the sources of the observed behavior.

Cycle-to-cycle variations in internal combustion engines are known to lead to limitations in engine load and efficiency, as well as increases in emissions. Recent research has led to the identification of the source of cyclic variations of pressure, soot and NO emissions in direct injection common rail diesel engines, when employing a single block injection and operating under long ignition delay conditions. The variations in peak pressure arise from changes in the diffusion combustion rate, caused by randomly occurring in-cylinder pressure fluctuations. These fluctuations result from the excitation of the first radial mode of vibration of the cylinder gases which arises from the rapid premixed combustion after the long ignition delay period. Cycles with high-intensity fluctuations present faster diffusion combustion, resulting in higher cycle peak pressure, as well as higher measured exhaust NO concentrations.

Past research has shown that post injections have the potential to reduce Diesel engine exhaust PM concentration without any significant influence in NOx emissions. However, an accurate, widely applicable rule of how to parameterize a post injection such that it provides a maximum reduction of PM emissions does not exist. Moreover, the underlying mechanisms are not thoroughly understood. In past research, the underlying mechanisms have been investigated in engine experiments, in constant volume chambers and also using detailed 3D CFD-CMC simulations. It has been observed that soot reduction due to a post injection is mainly due to two reasons: increased turbulence from the post injection during soot oxidation and lower soot formation due to lower amount of fuel in the main combustion at similar load conditions. Those studies do not show a significant temperature rise caused by the post injection.

A detailed chemical model was implemented in the KIVA-3V two dimensional CFD code to investigate the effects of the spray cone angle and injection timing on the PCCI combustion process and emissions in an optical research diesel engine. A detailed chemical model for Primary Reference Fuel (PRF) consisting of 157 species and 1552 reactions was used to simulate diesel fuel chemistry. The model validation shows good agreement between the predicted and measured pressure and emissions data in the selected cases with various spray angles and injection timings. If the injection is retarded to -50° ATDC, the spray impingement at the edge of the piston corner with 100° injection angle was shown to enhance the mixing of air and fuel. The minimum fuel loss and more widely distributed fuel vapor contribute to improving combustion efficiency and lowering uHC and CO emissions in the engine idle condition.

In this study we classify established and possible future engine combustion systems according to two main criteria, i.e. charge preparation (homogeneous or stratified) and type of combustion initiation (external, typically spark ignition and internal, typically due to compression). We discuss the relevant pros and cons of the four resulting energy conversion processes with emphasis on combustion stability, thermal efficiency and pollutant emissions. We show thereby that these output parameters are dominated by specific thermochemical and fluiddynamic processes as well as their complex interaction within the time scales of a thermodynamically optimal energy conversion at a given engine speed and load. For unsteady operation in mobile applications, the complexity of new combustion concepts may, nevertheless, prevent a breakthrough, despite their in-principle attractivity.

The spray development of ethanol, gasoline and iso-octane has been studied in an optically accessible, spark-ignition direct-injection (SIDI) engine. The focus is on how fuel properties impact temporal and spatial evolution of sprays at realistic ambient conditions. Two optical facilities were used: (1) a constant-flow spray chamber simulating cold-start conditions and (2) a single-cylinder SIDI engine running at normal, warmed-up operating conditions. In these optical facilities, high-speed Mie-scattering imaging is performed to measure penetrations of spray plumes at various injection pressures of 4, 7, 11 and 15 MPa. The results show that the effect of fuel type on the tip penetration length of the sprays depends on the injection conditions and the level of fuel jet atomisation and droplet breakup.

The operation of dual fuel engines, operated with natural gas as main fuel, offers the potential of substantial savings in CO2. Nevertheless, the operating map area where low pollutant emissions are produced is very narrow. Especially at low load, the raw exhaust gas contains high concentrations of unburned methane and, with high pilot fuel portions due to ignition limitations, also soot. The analysis of the combustion in those conditions in particular is not trivial, since multiple combustion modes are present concurrently. The present work focuses on the evaluation of the individual combustion modes of a dual fuel engine, operated with natural gas as main and diesel as pilot fuel, using a combustion model. The combustion has been split in two partwise concurrent combustion phases: the auto-ignition phase and the premixed flame propagation phase.

Future fuels will come from a variety of feed stocks and refinement processes. Understanding the fundamentals of combustion and pollutants formation of these fuels will help clear hurdles in developing flex-fuel combustors. To this end, we investigated the combustion, soot formation, and soot oxidation processes for various classes of fuels, each with distinct physical properties and molecular structures. The fuels considered include: conventional No. 2 diesel (D2), low-aromatics jet fuel (JC), world-average jet fuel (JW), Fischer-Tropsch synthetic fuel (JS), coal-derived fuel (JP), and a two-component surrogate fuel (SR). Fuel sprays were injected into high-temperature, high-pressure ambient conditions that were representative of a practical diesel engine. Simultaneous laser extinction measurement and planar laser-induced incandescence imaging were performed to derive the in-situ soot volume fraction.

Numerical simulations of soot formation were performed for n-dodecane spray using the transported probability density function (TPDF) method. Liquid n-dodecane was injected with 1500 bar fuel pressure into a constant-volume vessel with an ambient temperature, oxygen volume fraction and density of 900 K, 15% and 22.8 kg/m3, respectively. The interaction by exchange with the mean (IEM) model was employed to close the micro-mixing term. The unsteady Reynolds-averaged Navier-Stokes (RANS) equations coupled with the realizable k-ε turbulence model were used to provide turbulence information to the TPDF solver. A 53-species reduced n-dodecane chemical mechanism was employed to evaluate the reaction rates. Soot formation was modelled with an acetylene-based two-equation model which accounts for simultaneous soot particle inception, surface growth, coagulation and oxidation by O2 and OH.