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The stochastic pre-ignition phenomenon plays a vital role to limit the further increasing BMEP for natural gas engines. In this study, the pre-ignition propensities were examined in a highly boosted premixed natural gas engine by various engine loads and air/fuel ratios, as well as different methane number (MN) altered by hydrogen addition. A proper pre-ignition evaluation method was proposed referring to intake temperature. Moreover, the limits of in-cylinder temperature and pressure for the onset of pre-ignition were estimated. The results show that both higher IMEP and richer mixture conditions readily lead to pre-ignition. The significant increases of pre-ignition frequency and heavy-knocking pre-ignition cycle present with lowering MN.