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For the improvement of the vehicle yaw stability, this paper studies the control problem of the active front steering (AFS) system with actuator input delay. A novel sliding mode predictive control method to handle actuator input delay is proposed for the AFS system. Firstly, considering the nonlinearities of the vehicle system, a linear parameter varying vehicle system model with two-level structure is proposed to capture the vehicle dynamic behaviors. Secondly, to deal with the issues of actuator input delay and system constraints, a novel sliding mode predictive control method is put forward. In the process of controller design, a sliding mode control algorithm is employed for the improvement of the robustness of the control system, and then a model predictive control algorithm is employed to deal with system constraints.