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There is keen interest in understanding the origins of engine-out unburned hydrocarbons emitted during SI engine cold start. This is especially true for the first few firing cycles, which can contribute disproportionately to the total emissions measured over standard drive cycles such as the US Federal Test Procedure (FTP). This study reports on the development of a novel methodology for capturing and quantifying unburned hydrocarbon emissions (HC), CO, and CO2 on a cycle-by-cycle basis during an engine cold start. The method was demonstrated by applying it to a 4 cylinder 2 liter GTDI (Gasoline Turbocharged Direct Injection) engine for cold start conditions at an ambient temperature of 22°C. For this technique, the entirety of the engine exhaust gas was captured for a predetermined number of firing cycles.

A spontaneous Raman scattering diagnostic was used to measure the residual fraction in a single-cylinder, 4-valve optically accessible engine. The engine was operated at 1500 rpm on pre-vaporized iso-octane at several intake manifold pressures (50-90 kPa). Cam phasing was varied to determine the effect of intake valve timing and valve overlap on the residual mass fraction of the engine. A simple model based on the ideal Otto cycle and 1D gas flow through the exhaust valves was proposed to analyze the results of the Raman experiment. The model showed good agreement (R2=0.91) with the experimental results and demonstrated its potential for use as a method to estimate the residual fraction in an engine from available dynamometer data. The experimental results showed that the residual fraction was reduced at higher manifold pressures due to less backflow through the exhaust valves and varied with intake cam phasing.