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This work is a continuation of earlier results presented by the authors. In the current investigations the biofuels hydrogenated vegetable oil (HVO) and 1-octanol are investigated as pure components and compared to EN 590 Diesel. In a final step both biofuels are blended together in an appropriate ratio to tailor the fuels properties in order to obtain an optimal fuel for a clean combustion. The results of pure HVO indicate a significant reduction in CO-, HC- and combustion noise emissions at constant NOX levels. With regard to soot emissions, at higher part loads, the aromatic free, paraffinic composition of HVO showed a significant reduction compared to EN 590 petroleum Diesel fuel. But at lower loads the high cetane number leads to shorter ignition delays and therefore, ignition under richer conditions.

Combustion and pollutant formation in a new recently introduced Common-Rail DI Diesel engine concept with roof-shaped combustion chamber and tumble charge motion are numerically investigated using the Representative Interactive Flamelet concept (RIF). A reference case with a cup shaped piston bowl for full load operating conditions is considered in detail. In addition to the reference case, three more cases are investigated with a variation of start of injection (SOI). A surrogate fuel consisting of n-decane (70% liquid volume fraction) and α-methylnaphthalene (30% liquid volume fraction) is used in the simulation. The underlying complete reaction mechanism comprises 506 elementary reactions and 118 chemical species. Special emphasis is put on pollutant formation, in particular on the formation of NOx, where a new technique based on a three-dimensional transport equation within the flamelet framework is applied.

Within the Cluster of Excellence “Tailor-Made Fuels from Biomass” (TMFB) at the RWTH Aachen University, two novel biogenic fuels, namely 1-octanol and its isomer dibutyl ether (DBE), were identified and extensively analyzed in respect of their suitability for combustion in a Diesel engine. Both biofuels feature very different properties, especially regarding their ignitability. In previous works of the research cluster, promising synthesis routes with excellent yields for both fuels were found, using lignocellulosic biomass as source material. Both fuels were investigated as pure components in optical and thermodynamic single cylinder engines (SCE). For 1-octanol at lower part load, almost no soot emission could be measured, while with DBE the soot emissions were only about a quarter of that with conventional Diesel fuel. At high part load (2400 min-1, 14.8 bar IMEP), the soot reduction of 1-octanol was more than 50% and for DBE more than 80 % respectively.

Within this paper, the two possible alternative and biomass-based fuel candidates Di-n-butyl ether (DNBE) and 1-octanol are investigated with regard to their utilization in a diesel-type engine. In order to asses the fuels emission-reduction potential, both have been tested in a single cylinder engine (SCE) and a high pressure chamber (HPC) in comparison to conventional EN590 diesel at various load points. Due to its reduced reactivity 1-octanol features a longer ignition delay and thus higher degrees of homogenization at start of combustion, whereas DNBE ignites rather rapidly in both the HPC and the engine leading to a predominantly mixing controlled combustion. Thus, both fuels feature completely different combustion characteristics. However, compared to diesel, both fuels contribute to a significant reduction in Filter Smoke Number (FSN) up to a factor of 15.

Due to experimental challenges, combustion of diesel-like jets has rarely been characterized by laser-based quantitative multiscalar measurements. In this work, recently developed laser diagnostics for combustion temperature and the concentrations of CO, O2, and NO are applied to a diesel-like jet, using a highly oxygenated fuel. The diagnostic is based on spontaneous Raman scattering (SRS) and laser-induced fluorescence (LIF) methods. Line imaging yields multiscalar profiles across the jet cross section. Measurements turn out to be particularly accurate, because near-stoichiometric combustion occurs in the central region of the jet. Thereby, experimental cross-influences by light attenuation and interfering emissions are greatly reduced compared to the combustion of conventional, sooting diesel fuel jets. This is achieved by fuel oxygenation and enhanced premixing.

The influence of different fuels and injection pressures on the flame lift-off length (LOL), as well as the combustion structure under quiescent conditions in a heated high-pressure vessel were experimentally investigated using OH chemiluminescence measurements. This data was used to validate the newly developed G-equation coupled with MRIF (G-MRIF) model, which was designed to describe the lifted Diesel combustion process. The achieved results are very promising and could be used as a tool to apply this combustion mode into Diesel engines. Furthermore these measurements were used to validate the approach of a new combustion model, which was developed using former OH chemiluminescence measurements by the authors. Based on this approach the LOL is mainly determined by auto-ignition and therefore highly dependent on the cetane number. This model is presented in more detail within this work.

Current and future emission legislations require a significant reduction of engine-out emissions for Diesel engines. For a further reduction of engine-out emissions, different measures are necessary such as: Especially an advanced emission and closed-loop combustion control has gained increased significance during the past years.

In order to reduce engine out CO2 emissions it is a main subject to find new alternative fuels out of renewable sources. For this paper, several fuels were selected which can be produced out of biomass or with hydrogen which is generated directly via electrolysis with electricity from renewable sources. All fuels are compared to conventional diesel fuel and two diesel surrogates. It is well known that there can be a large effect of fuel properties on mixture formation and combustion, which may result in a completely different engine performance compared to the operation with conventional diesel fuels. Mixture formation and ignition behavior can also largely affect the pollutant formation. The knowledge of the combustion behavior is also important to design new engine geometries or implement new calibrations for an existing engine. The fuel properties of the investigated fuels comprise a large range, for example in case of the derived cetane number, from below 30 up to 100.

Within this study a dual-fuel concept was experimentally investigated. The utilized fuels were conventional EN228 RON95E10 and EN590 Diesel B7 pump fuels. The engine was a single cylinder Diesel research engine for passenger car application. Except for the installation of the port fuel injection valve, the engine was not modified. The investigated engine load range covered low part load operation of IMEP = 4.3 bar up to IMEP = 14.8 bar at different engine speeds. Investigations with Diesel pilot injection showed that the dual-fuel approach can significantly reduce the soot/NOx-trade-off, but typically increases the HC- and CO-emissions. At high engine load and gasoline mass fraction, the premixed gasoline/air self-ignited before Diesel fuel was injected. Reactivity Controlled Compression Ignition (RCCI) was subsequently investigated in a medium load point at IMEP = 6.8 bar.

To comply with the new regulations on particulate matter emissions, the manufacturers of light-duty as well as heavy-duty vehicles more commonly use diesel particulate filters (DPF). The regeneration of DPF depends to a significant extent on the properties of the soot stored. Within the Cluster of Excellence "Tailor-Made Fuels from Biomass (TMFB)" at RWTH Aachen University, the Institute for Combustion Engines carried out a detailed investigation program to explore the potential of future biofuel candidates for optimized combustion systems. The experiments for particulate measurements and analysis were conducted on a EURO 6-compliant High Efficiency Diesel Combustion System (HECS) with petroleum-based diesel fuel as reference and a today's commercial biofuel (i.e., FAME) as well as a potential future biomass-derived fuel candidate (i.e., 2-MTHF/DBE). Thermo gravimetric analyzer (TGA) was used in this study to evaluate the oxidative reactivity of the soot.

Tightening of emission norms necessitate intensified research in the field of emissions reduction. Fuel research opens up a vast area of potential improvement, since combustion behavior and the nature of the combustion products can be heavily influenced by fuel composition. In this paper, the effects of fuel properties on combustion and emissions shall be discussed, based on the study of standard diesel fuel, two types of diesel-like fuels and a kerosene fuel. Investigations were conducted on a single cylinder heavy duty direct-injected diesel engine operating under part-homogeneous combustion in the part-load operating range. For this purpose, a statistical design of experiments method (DOE) was utilized in order to evaluate the influence of each fuel property and, thus, develop a model for all selected fuels. Variation in EGR rates, injection and air patterns have significant effects on the combustion in the fuels under investigation.

Partly homogeneous combustion (PHC) can assist the reduction of the engine-out emissions but its influence is limited by using conventional diesel fuel. To verify whether alternatively designed fuels can help to improve the PHC performance, the impact of different fuel properties in combination with engine control levers have been studied. Based on single cylinder heavy duty direct injection diesel engine (DIDE) test results with different diesel and diesel-like fuels, operating under partly homogeneous combustion conditions, the impact of the combination of the fuel properties were investigated. The fuel matrix was designed such that the fuel properties varied in sufficiently large ranges, in order to be able to detect the impact of the properties at the selected operating points. A statistical principal component analysis (PCA) has been applied to the fuel matrix to specify the interrelationship between the fuel properties, as well as to derive the most independent fuel properties.

The influence of two oxygenated tailor-made fuels on soot formation and oxidation in an optical single cylinder research diesel engine has been studied. For the investigation a planar laser-induced incandescence (PLII) measurement technique was applied to the engine in order to detect and evaluate the planar soot distribution for the two bio fuels within a laser light sheet. Furthermore the OH* chemiluminescence and broad band soot luminosity was visualized by high speed imaging to compare the ignition and combustion behavior of tested fuels: Two C8 oxygenates, di-n-butylether (DNBE) and 1-octanol. Both fuels have the same molecular formula but differ in their molecular structure. DNBE ignites fast and burns mostly diffusive while 1-octanol has a low cetane number and therefore it has a longer ignition delay but a more homogeneous mixture at time of ignition. The two bio fuels were finally compared to conventional diesel fuel.

Oxygenated fuels such as polyoxymethylene dimethyl ethers (OME) offer a chance to significantly decrease emissions while switching to renewable fuels. However, compared to conventional diesel fuel, they have lower heating values and different evaporation behaviors which lead to differences in spray, mixture formation as well as ignition delay. In order to determine the mixture formation characteristics and the combustion behavior of neat OME3-5, optical investigations have been carried out in a high-pressure-chamber using shadowgraphy, mie-scatterlight and OH-radiation recordings. Liquid penetration length, gaseous penetration length, lift off length, spray cone angle and ignition delay have been determined and compared to those measured with diesel-fuel over a variety of pressures, temperatures, rail pressures and injection durations.

The finite nature and instability of fossil fuel supply has led to an increasing and enduring investigation demand of alternative and regenerative fuels. An investigation program is carried out to explore the potential of tailor made fuels to reduce engine-out emissions while maintaining engine efficiency and an acceptable noise level. In this paper, fundamental results of the Diesel engine relevant combustion are presented. To enable optimum engine performance a range of different reference fuels have been investigated. The fundamental effects of different physical and chemical properties on emission formation and engine performance are investigated using a thermodynamic diesel single cylinder research engine and an optically-accessible combustion vessel. Depending on the chain length and molecular structure, fuel compounds vary in cetane number, boiling temperature etc. Therefore, different hydrocarbons including n-heptane, n-dodecane, and l-decanol were investigated.

Modern biofuels offer the potential to decrease engine out emissions while at the same time contributing to a reduction of greenhouse gases produced from individual mobility. In order to deeply investigate and improve the complete path from biofuel production to combustion, in 2007 the cluster of excellence “Tailor-Made Fuels from Biomass” was installed at RWTH Aachen University. Since then, a whole variety of possible fuel candidates have been identified and investigated. In particular oxygenated fuels (e.g. alcohols, furans) have proven to be beneficial regarding the particulate matter (PM)/ NOx trade-off [1, 2, 3] in diesel-type combustion. Alcohols that provide a longer ignition delay than diesel might behave even better with regard to this trade-off due to higher homogenization of the mixture. Recent studies carried out within the Cluster of Excellence have discovered new pathways to derive 1-octanol from biomass [4], which features a derived cetane number (DCN) of 39.

If fuels that are more resistant to auto-ignition are injected near TDC in compression ignition engines, they ignite much later than diesel fuel and combustion occurs when the fuel and air have had more chance to mix. This helps to reduce NOX and smoke emissions at much lower injection pressures compared to a diesel fuel. However, PPCI (Partially Premixed Compression Ignition) operation also leads to higher CO and HC at low loads and higher heat release rates at high loads. These problems can be significantly alleviated by managing the mixing through injector design (e.g. nozzle size and centreline spray angle) and changing CR (Compression Ratio). This work describes results of running a single-cylinder diesel engine on fuel blends by using three different nozzle design (nozzle size: 0.13 mm and 0.17 mm, centreline spray angle: 153° and 120°) and two different CRs (15.9:1 and 18:1).

Lignocellulosic biomass consists of (hemi-) cellulose and lignin. Accordingly, an integrated biorefinery will seek to valorize both streams into higher value fuels and chemicals. To this end, this study evaluated the overall combustion performance of both cellulose- and lignin derivatives, namely the high cetane number (CN) di-n-butyl ether (DnBE) and low CN anisole, respectively. Said compounds were blended both separately and together with EN590 diesel. Experiments were conducted in a single cylinder compression ignition engine, which has been optimized for improved combustion characteristics with respect to low emission levels and at the same time high fuel efficiency. The selected operating conditions have been adopted from previous “Tailor-Made Fuels from Biomass (TMFB)” work.

Today's biofuels require large amounts of energy in the production process for the conversion from biomass into fuels with conventional properties. To reduce the amounts of energy needed, future fuels derived from biomass will have a molecular structure which is more similar to the respective feedstock. Butyl levulinate can be gained easily from levulinic acid which is produced by acid hydrolysis of cellulose. Thus, the Institute for Combustion Engines at RWTH Aachen University carried out a fuel investigation program to explore the potential of this biofuel compound, as a candidate for future compression ignition engines to reduce engine-out emissions while maintaining engine efficiency and an acceptable noise level. Previous investigations identified most desirable fuel properties like a reduced cetane number, an increased amount of oxygen content and a low boiling temperature for compression ignition engine conditions.

The limited availability of fossil fuels and the increasing environmental pollution will lead to an increased demand for sustainable biofuels. The production of bio-based diesel fuels from vegetable oils is commonly accomplished using a process known as Trans-esterification. The product of Transesterification is Fatty Acid Methyl Ester (FAME), commonly known as Biodiesel. An alternative process is Hydro-treatment of seed oils or animal waste fats to produce highly paraffinic renewable diesel fuel called Hydrogenated Vegetable Oil (HVO). Detailed investigations were carried out by the “Department of Advanced Diesel Engine Development” at FEV GmbH Aachen (Germany), to explore the potential of this biofuel compound as a candidate for future compression ignition engines.