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Laser excitation wavelengths for two-line planar laser-induced fluorescence (PLIF) of 3-pentanone have been optimized for simultaneous imaging of temperature and composition under engine-relevant conditions. Validation of the diagnostic was performed in a motored optical IC engine seeded homogeneously with 3-pentanone. PLIF measurements of the uniform mixture during the compression stroke were used to measure the average temperature and to access the random uncertainty in the measurements. To determine the accuracy of the temperature measurements, experimental average temperatures were compared to values computed assuming isentropic compression and to the output of a tuned 1-D engine simulation. The comparison indicated that the absolute accuracy of the temperature measurements is better than ±5%. Probability density functions (PDFs) calculated from the single-shot images were used to estimate the precision of the measurements.

Many experimental efforts to track fuel-air-residual mixture preparation in internal combustion engines have employed laser induced fluorescence (LIF) of tracers. Acetone and 3-pentanone are often chosen as tracers because of their relatively strong LIF signal, weak quenching, and reasonable match to thermo-chemical properties of common fuels such as iso-octane. However, the addition of these tracers to fuel-air mixtures could affect combustion behavior. In this work, we assess these effects to better understand limitations of tracer-based engine measurements. The effects of tracer seeding on combustion phasing, duration, and variation are studied in an HCCI engine using a recompression strategy to accommodate single- and multi-stage-ignition fuels.

Negative valve overlap (NVO) is a valve strategy employed to retain and recompress residual burned gases to assist HCCI combustion, particularly in the difficult regime of low-load operation. NVO allows the retention of large quantities of hot residual burned gases as well as the possibility of fuel addition for combustion control purposes. Reaction of fuel injected during NVO increases charge temperature, but in addition could produce reformed fuel species that may affect main combustion phasing. The strategy holds potential for controlling and extending low-load HCCI combustion. The goal of this work is to demonstrate the feasibility of applying two-wavelength PLIF of 3-pentanone to obtain simultaneous, in-cylinder temperature and composition images during different parts of the HCCI/NVO cycle. Measurements are recorded during the intake and main compression strokes, as well as during the more challenging periods of NVO recompression and re-expansion.