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Long chain alcohols possess major advantages over the currently used ethanol as bio-components for gasoline, including higher energy content, better engine compatibility, and less water solubility. The rapid developments in biofuel technology have made it possible to produce C 4 -C 5 alcohols cost effectively. These higher alcohols could significantly expand the biofuel content and potentially substitute ethanol in future gasoline mixtures. This study characterizes some fundamental properties of a C 5 alcohol, isopentanol, as a fuel for HCCI engines. Wide ranges of engine speed, intake temperature, intake pressure, and equivalence ratio are investigated. Results are presented in comparison with gasoline or ethanol data previously reported. For a given combustion phasing, isopentanol requires lower intake temperatures than gasoline or ethanol at all tested speeds, indicating a higher HCCI reactivity.

An infrared laser absorption technique has been developed to measure in-cylinder concentrations of CO in an optical, automotive HCCI engine. The diagnostic employs a distributed-feedback, tunable diode laser selected to emit light at the R15 line of the first overtone of CO near 2.3 μm. The collimated laser beam makes multiple passes through the cylinder to increase its path length and its sampling volume. High-frequency modulation of the laser output (wavelength modulation spectroscopy) further enhances the signal-to-noise ratio and detection limits of CO. The diagnostic has been tested in the motored and fired engine, exhibiting better than 200-ppm sensitivity for 50-cycle ensemble-average values of CO concentration with 1-ms time resolution. Fired results demonstrate the ability of the diagnostic to quantify CO production during negative valve overlap (NVO) for a range of fueling conditions.

The potential of boosted HCCI for achieving high loads has been investigated for intake pressures (Piⁿ) from 100 kPa (naturally aspirated) to 325 kPa absolute. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) equipped with a compression-ratio 14 piston at 1200 rpm. The intake charge was fully premixed well upstream of the intake, and the fuel was a research-grade (R+M)/2 = 87-octane gasoline with a composition typical of commercial gasolines. Beginning with Piⁿ = 100 kPa, the intake pressure was systematically increased in steps of 20 - 40 kPa, and for each Piⁿ, the fueling was incrementally increased up to the knock/stability limit, beyond which slight changes in combustion conditions can lead to strong knocking or misfire. A combination of reduced intake temperature and cooled EGR was used to compensate for the pressure-induced enhancement of autoignition and to provide sufficient combustion-phasing retard to control knock.

One in-cylinder strategy for reducing soot emissions from diesel engines while maintaining fuel efficiency is the use of close-coupled post injections, which are small fuel injections that follow the main fuel injection after a short delay. While the in-cylinder mechanisms of diesel combustion with single injections have been studied extensively and are relatively well understood, the in-cylinder mechanisms affecting the performance and efficacy of post injections have not been clearly established. Here, experiments from a single-cylinder heavy-duty optical research engine incorporating close- coupled post injections are modeled with three dimensional (3D) computational fluid dynamics (CFD) simulations. The overall goal is to complement experimental findings with CFD results to gain more insight into the relationship between post-injections and soot. This paper documents the first stage of CFD results for simulating and analyzing the experimental conditions.

Negative valve overlap (NVO) is an operating mode that enables efficient, low-temperature gasoline combustion in automotive engines. In addition to retaining a large fraction of residuals, NVO operation also enables partial fuel injection during the recompression period as a means of enhancing and controlling main combustion. Thermal effects of NVO fueling on main combustion are well understood, but chemical effects of the products of NVO reactions remain uncertain. To address this topic, we have fabricated a dump valve that extracts a large fraction of cylinder charge at intake valve closing (IVC), yielding a representative sample of NVO products mixed with intake air. Sample composition is determined by gas chromatography. Results from a sweep of NVO start-of-injection (SOI) timings show that concentrations of the reactive species acetylene and hydrogen rise to several hundred parts-per-million as NVO SOI is retarded toward top center of NVO.

One way to increase the load range in an HCCI engine is to increase boost pressure. In this modeling study, we investigate the effect of increased boost pressure on the fuel chemistry in an HCCI engine. Computed results of HCCI combustion are compared to experimental results in a HCCI engine. We examine the influence of boost pressure using a number of different detailed chemical kinetic models - representing both pure compounds (methylcyclohexane, cyclohexane, iso-octane and n-heptane) and multi-component models (primary reference fuel model and gasoline surrogate fuel model). We examine how the model predictions are altered by increased fueling, as well as reaction rate variation, and the inclusion of residuals in our calculations. In this study, we probe the low temperature chemistry (LTC) region and examine the chemistry responsible for the low-temperature heat release (LTHR) for wide ranges of intake boost pressure.

Laser excitation wavelengths for two-line planar laser-induced fluorescence (PLIF) of 3-pentanone have been optimized for simultaneous imaging of temperature and composition under engine-relevant conditions. Validation of the diagnostic was performed in a motored optical IC engine seeded homogeneously with 3-pentanone. PLIF measurements of the uniform mixture during the compression stroke were used to measure the average temperature and to access the random uncertainty in the measurements. To determine the accuracy of the temperature measurements, experimental average temperatures were compared to values computed assuming isentropic compression and to the output of a tuned 1-D engine simulation. The comparison indicated that the absolute accuracy of the temperature measurements is better than ±5%. Probability density functions (PDFs) calculated from the single-shot images were used to estimate the precision of the measurements.

This work explores the high-load limits of HCCI for naturally aspirated operation. This is done for three fuels with various autoignition reactivity: iso-octane, PRF80, and PRF60. The experiments were conducted in a single-cylinder HCCI research engine (0.98 liter displacement), mostly with a CR = 14 piston installed, but with some tests at CR = 18. Five load-limiting factors were identified: 1) NOx-induced combustion-phasing run-away, 2) wall-heating-induced run-away, 3) EGR-induced oxygen deprivation, 4) wandering unsteady combustion, and 5) excessive exhaust NOx. These experiments at 1200 rpm show that the actual load-limiting factor is dependent on the autoignition reactivity of the fuel, the selected CA50, and in some cases, the tolerable level of NOx emissions. For iso-octane, which has the highest resistance to autoignition of the fuels tested, the NOx emissions become unacceptable at IMEPg = 473 kPa.

This paper investigates flow and combustion in a full-cycle simulation of a four-stroke, three-valve HCCI engine by visualizing the flow with pathlines. Pathlines trace massless particles in a transient flow field. In addition to visualization, pathlines are used here to trace the history, or evolution, of flow fields and species. In this study evolution is followed from the intake port through combustion. Pathline analysis follows packets of intake charge in time and space from induction through combustion. The local scalar fields traversed by the individual packets in terms of velocity magnitude, turbulence, species concentration and temperatures are extracted from the simulation results. The results show how the intake event establishes local chemical and thermal environments in-cylinder and how the species respond (chemically react) to the local field.

A planar temperature imaging diagnostic has been developed and applied to an investigation of naturally occurring thermal stratification in an HCCI engine. Natural thermal stratification is critical for high-load HCCI operation because it slows the combustion heat release; however, little is known about its development or distribution. A tracer-based single-line PLIF imaging technique was selected for its good precision and simplicity. Temperature-map images were derived from the PLIF images, based on the temperature sensitivity of the fluorescence signal of the toluene tracer added to the fuel. A well premixed intake charge assured that variations in fuel/air mixture did not affect the signal. Measurements were made in a single-cylinder optically accessible HCCI research engine (displacement = 0.98 liters) at a typical 1200 rpm operating condition. Since natural thermal stratification develops prior to autoignition, all measurements were made for motored operation.

Negative valve overlap (NVO) is a valve strategy employed to retain and recompress residual burned gases to assist HCCI combustion, particularly in the difficult regime of low-load operation. NVO allows the retention of large quantities of hot residual burned gases as well as the possibility of fuel addition for combustion control purposes. Reaction of fuel injected during NVO increases charge temperature, but in addition could produce reformed fuel species that may affect main combustion phasing. The strategy holds potential for controlling and extending low-load HCCI combustion. The goal of this work is to demonstrate the feasibility of applying two-wavelength PLIF of 3-pentanone to obtain simultaneous, in-cylinder temperature and composition images during different parts of the HCCI/NVO cycle. Measurements are recorded during the intake and main compression strokes, as well as during the more challenging periods of NVO recompression and re-expansion.

Tracer-based PLIF temperature diagnostics have been used to study the distribution and evolution of naturally occurring thermal stratification (TS) in an HCCI engine under fired and motored operation. PLIF measurements, performed with two excitation wavelengths (277, 308 nm) and 3-pentanone as a tracer, allowed investigation of TS development under relevant fired conditions. Two-line PLIF measurements of temperature and composition were first performed to track the mixing of the fresh charge and hot residuals during intake and early compression strokes. Results showed that mixing occurs rapidly with no measureable mixture stratification remaining by early compression (220°CA aTDC), confirming that the residual mixing is not a leading cause of thermal stratification for low-residual (4-6%) engines with conventional valve timing.

Isopentanol is an advanced biofuel that can be produced by micro-organisms through genetically engineered metabolic pathways. Compared to the more frequently studied ethanol, isopentanol's molecular structure has a longer carbon chain and includes a methyl branch. Its volumetric energy density is over 30% higher than ethanol, and it is less hygroscopic. Some fundamental combustion properties of isopentanol in an HCCI engine have been characterized in a recent study by Yang and Dec (SAE 2010-01-2164). They found that for typical HCCI operating conditions, isopentanol lacks two-stage ignition properties, yet it has a higher HCCI reactivity than gasoline. The amount of intermediate temperature heat release (ITHR) is an important fuel property, and having sufficient ITHR is critical for HCCI operation without knock at high loads using intake-pressure boosting. Isopentanol shows considerable ITHR, and the amount of ITHR increases with boost, similar to gasoline.

This study investigates the potential of partial fuel stratification for reducing the knocking propensity of intake-boosted HCCI engines operating on conventional gasoline. Although intake boosting can substantially increase the high-load capability of HCCI, these engines would be more production-viable if the knock/stability load limit could be extended to allow higher loads at a given boost and/or to provide even higher thermal efficiencies. A technique termed partial fuel stratification (PFS) has recently been shown to greatly reduce the combustion-induced pressure-rise rate (PRR), and therefore the knocking propensity of naturally aspirated HCCI, when the engine is fueled with a φ-sensitive, two-stage-ignition fuel. The current work explores the potential of applying PFS to boosted HCCI operation using conventional gasoline, which does not typically show two-stage ignition. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) at 1200 rpm.

A tracer-based single-line PLIF imaging technique using a unique optical configuration that allows simultaneously viewing the bulk-gas and the boundary layer region has been applied to an investigation of the naturally occurring thermal stratification in a HCCI engine. Thermal stratification is critical for HCCI engines, because it determines the maximum pressure rise rate which is a limiting factor for high-load operation. The investigation is based on the analysis of temperature maps that were derived from PLIF images, using the temperature sensitivity of fluorescence from toluene introduced as tracer in the fuel. Measurements were made in a single-cylinder optically accessible HCCI engine operating under motored conditions with a vertical laser-sheet orientation that allows observation of the development of thermal stratification from the cold boundary layers into the central region of the charge.

Prior studies have shown that fuel addition during negative valve overlap (NVO) can both increase temperature and alter composition of the charge carried over to main HCCI combustion. Late NVO fuel injection, i.e., near top dead center, can cause piston wetting and subsequent localized rich flames. Since acetylene is a product of rich combustion and is known to advance ignition, it is hypothesized that the species could play a chemical role in enhancing main combustion. The objective of this work is to quantify the effects of acetylene on HCCI combustion. While the research topic is specifically relevant to NVO-fueled HCCI operation, the experiments are conducted without NVO fueling to avoid uncertainties of NVO reforming reactions. Instead, a single post-NVO injection of iso-octane fuels the cycle, and acetylene is seeded into the intake flow at varying concentrations to simulate a reformed product of NVO.

Laser-induced incandescence (LII) has been explored as a diagnostic for qualitative two-dimensional imaging of the in-cylinder soot distribution in a diesel engine. Advantages of LII over elastic-scatter soot imaging techniques include no interfering signals from liquid fuel droplets, easy rejection of laser light scattered by in-cylinder surfaces, and the signal intensity being proportional to the soot volume fraction. LII images were obtained in a 2.3-liter, single cylinder, direct-injection diesel engine, modified for optical access. To minimize laser sheet and signal attenuation (which can affect almost any planar imaging technique applied to diesel engine combustion), a low-sooting fuel was used whose vaporization and combustion characteristics are typical of standard diesel fuels. Temporal and spatial sequences of LII images were made which show the extent of the soot distribution within the optically accessible portion the combusting spray plume.

Ethanol and ethanol/gasoline blends are being widely considered as alternative fuels for light-duty automotive applications. At the same time, HCCI combustion has the potential to provide high efficiency and ultra-low exhaust emissions. However, the application of HCCI is typically limited to low and moderate loads because of unacceptably high heat-release rates (HRR) at higher fueling rates. This work investigates the potential of lowering the HCCI HRR at high loads by using partial fuel stratification to increase the in-cylinder thermal stratification. This strategy is based on ethanol's high heat of vaporization combined with its true single-stage ignition characteristics. Using partial fuel stratification, the strong fuel-vaporization cooling produces thermal stratification due to variations in the amount of fuel vaporization in different parts of the combustion chamber.

Fuel stratification has been investigated as a means of improving the low-load combustion efficiency in an HCCI engine. Several stratification techniques were examined: different GDI injectors, increased swirl, and changes in injection pressure, to determine which parameters are effective for improving the combustion efficiency while maintaining NOx emissions below U.S. 2010 limits. Performance and emission measurements were obtained in an all-metal engine. Corresponding fuel distribution measurements were made with fuel PLIF imaging in a matching optically accessible engine. The fuel used was iso-octane, which is a good surrogate for gasoline. For an idle fueling rate (ϕ = 0.12), combustion efficiency was improved substantially, from 64% to 89% at the NOx limit, using delayed fuel injection with a hollow-cone injector at an injection pressure of 120 bar.

NO formation during direct-injection (DI) diesel combustion has been investigated using planar laser-induced fluorescence (PLIF) imaging. Measurements were made at a typical medium-speed operating condition in a heavy-duty size-class engine modified for optical access. By combining a unique laser system with a particular spectroscopic scheme, single-shot NO images were obtained at realistic operating conditions with negligible O2 interference. Temporal sequences of NO PLIF images are presented along with corresponding images of combined elastic scattering and natural luminosity. These images show the location and timing of the NO formation relative to the other components of the reacting fuel jet. In addition, total NO formation was examined by integrating the NO PLIF signal over a large fraction of the combustion-chamber volume.