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Low temperature combustion (LTC) strategies, which can mitigate emissions of particulate matter (PM) and nitrogen oxides (NOx) from diesel engines, typically have longer ignition delays compared to conventional diesel operation. With extended ignition delays, more time is available for premixing, which reduces PM formation. The effect of varying ignition delay on the spatial and temporal evolution of soot in LTC diesel jets is studied by imaging the natural soot luminosity, while the in-cylinder soot mass and temperature are measured using two-color soot thermometry. Ignition delay in the engine is controlled by adjusting the intake air temperature while keeping the same charge density at TDC. This allowed us to study sooting characteristics at various ignition delays while keeping the same diesel jet penetration for all the cases.

The potential of boosted HCCI for achieving high loads has been investigated for intake pressures (Piⁿ) from 100 kPa (naturally aspirated) to 325 kPa absolute. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) equipped with a compression-ratio 14 piston at 1200 rpm. The intake charge was fully premixed well upstream of the intake, and the fuel was a research-grade (R+M)/2 = 87-octane gasoline with a composition typical of commercial gasolines. Beginning with Piⁿ = 100 kPa, the intake pressure was systematically increased in steps of 20 - 40 kPa, and for each Piⁿ, the fueling was incrementally increased up to the knock/stability limit, beyond which slight changes in combustion conditions can lead to strong knocking or misfire. A combination of reduced intake temperature and cooled EGR was used to compensate for the pressure-induced enhancement of autoignition and to provide sufficient combustion-phasing retard to control knock.

Low-temperature combustion (LTC) strategies for diesel engines are of increasing interest because of their potential to significantly reduce particulate matter (PM) and nitrogen oxide (NOx) emissions. LTC with late fuel injection further offers the benefit of combustion phasing control because ignition is closely coupled to the fuel injection event. But with a short ignition-delay, fuel jet mixing processes must be rapid to achieve adequate premixing before ignition. In the current study, mixing and pollutant formation of late-injection LTC are studied in a single-cylinder, direct-injection, optically accessible heavy-duty diesel engine using three laser-based imaging diagnostics. Simultaneous planar laser-induced fluorescence of the hydroxyl radical (OH) and combined formaldehyde (H2CO) and polycyclic aromatic hydrocarbons (PAH) are compared with vapor-fuel concentration measurements from a non-combusting condition.

A set of elementary surface reactions is proposed for modeling the chemistry in a lean NOx trap during regeneration (reduction of stored NOx). The proposed reaction mechanism can account for the observed product distribution from the trap over a range of temperatures and inlet gas compositions similar to those expected for realistic operation. The mechanism includes many reactions already discussed in the literature, together with some hypothesized reactions that are required to match observations from temperature programmed reactor experiments with a commercial lean NOx trap catalyst. Preliminary results indicate that the NOx trap regeneration and byproduct formation rates can be effectively captured by using a relatively compact set of elementary reactions.

Reaching for higher loads and improving combustion-phasing control are important challenges for HCCI research. Although HCCI engines can operate with a variety of fuels, recent research has shown that fuels with two-stage autoignition have some significant advantages for overcoming these challenges. Because the amount of low-temperature heat release (LTHR) is proportional to the local equivalence ratio (ϕ), fuel stratification can be used to adjust the combustion phasing (CA50) and/or burn duration using various fuel-injection strategies. Two-stage ignition fuels also allow stable combustion even for extensive combustion-phasing retard, which reduces the knocking propensity. Finally, the LTHR reduces the required intake temperature, which increases the inducted charge mass for a given intake pressure, allowing higher fueling rates before knocking and NOx emissions become a problem. However, the amount of LTHR is normally highly dependent on the engine speed.

Although low-temperature combustion (LTC) strategies for compression-ignition engines can achieve very low emissions of nitrogen oxides (NOx) and particulate matter (PM) at high efficiency, they typically have increased emissions of other pollutants, including unburned hydrocarbons (UHC). In the current study, the equivalence ratio of mixtures near the injector are quantified under non-combusting conditions by planar laser-Rayleigh scattering (PLRS) in a constant-volume combustion chamber and by planar laser-induced fluorescence (PLIF) of a fuel tracer (toluene) in a single-cylinder direct-injection heavy-duty diesel engine at typical LTC conditions. The optical diagnostic images show that the transient ramp-down at the end of fuel injection produces a low-momentum, fuel-lean mixture in the upstream region of the jet, which persists late in the cycle.

Methods of producing non-sooting, low flame temperature diesel combustion were investigated in an optically-accessible, quiescent constant-volume combustion vessel. Combustion and soot formation processes of single, isolated fuel jets were studied after autoignition and transient premixed combustion and while the injector needle was fully open (i.e., during the quasi-steady mixing-controlled phase of heat-release for diesel combustion).The investigation showed that fuel jets that do not undergo soot formation in any region of the reacting jet and that also have a low flame temperature could be produced in at least three different ways during mixing-controlled combustion: First, using a #2 diesel fuel and an injector tip with a 50 micron orifice, a fuel jet was non-sooting in ambient oxygen concentrations as low as 10% (simulating the use of EGR) for typical diesel ambient temperatures (1000 K) and densities.

The engine-out emissions and fuel consumption rates for a modern, heavy-duty diesel engine were compared when fueling with a conventional diesel fuel and three water-blend-fuel emulsions. Four different fuels were studied: (1) a conventional diesel fuel, (2) PuriNOx,™ a water-fuel emulsion using the same conventional diesel fuel, but having 20% water by mass, and (3,4) two other formulations of the PuriNOx™ fuel that contained proprietary chemical additives intended to improve combustion efficiency and emissions characteristics. The emissions data were acquired with three different injection-timing strategies using the AVL 8-Mode steady-state test method in a Caterpillar 3176 engine, which had a calibration that met the 1998 nitrogen oxides (NOX) emissions standard.

Significant reductions of particulate matter (PM) and nitrogen oxides (NOx) emissions from diesel engines have been realized through fueling with water-fuel emulsions. However, the physical and chemical in-cylinder mechanisms that affect these pollutant reductions are not well understood. To address this issue, laser-based and chemiluminescence imaging experiments were performed in an optically-accessible, heavy-duty diesel engine using both a standard diesel fuel (D2) and an emulsion of 20% water, by mass (W20). A laser-based Mie-scatter diagnostic was used to measure the liquid-phase fuel penetration and showed 40-70% greater maximum liquid lengths with W20 at the operating conditions tested. At some conditions with low charge temperature or density, the liquid phase fuel may impinge directly on in-cylinder surfaces, leading to increased PM, HC, and CO emissions because of poor mixing.

The combustion behavior of conventional gasoline has been numerically investigated by means of detailed chemical-kinetic modeling simulations, with particular emphasis on analyzing the chemistry of the intermediate temperature heat release (ITHR). Previous experimental work on highly boosted (up to 325 kPa absolute) HCCI combustion of gasoline (SAE 2020-01-1086) showed a steady increase in the charge temperature up to the point of hot ignition, even for conditions where the ignition point was retarded well after top dead center (TDC). Thus, sufficient energy was being released by early pre-ignition reactions resulting in temperature rise during the early part of the expansion stroke This behavior is associated with a slow pre-ignition heat release (ITHR), which is critical to keep the engine from misfiring at the very late combustion phasings required to prevent knock at high-load boosted conditions.

Three different approaches for modeling diesel engine combustion are compared against cylinder pressure, NOx emissions, high-speed soot luminosity imaging, and 2-color thermometry data from a heavy-duty DI diesel engine. A characteristic time combustion (KIVA-CTC) model, a representative interactive flamelet (KIVA-RIF) model, and direct integration using detailed chemistry (KIVA-CHEMKIN) were integrated into the same version of the KIVA-3v computer code. In this way, the computer code provides a common platform for comparing various combustion models. Five different engine operating strategies that are representative of several different combustion regimes were explored in the experiments and model simulations. Two of the strategies produce high-temperature combustion with different ignition delays, while the other three use dilution to achieve low-temperature combustion (LTC), with early, late, or multiple injections.

It is generally accepted that thermal (Zeldo'vich) chemical kinetics dominate NO formation in diesel engines, so control of temperature is critical for reducing exhaust NOx emissions. Recent optical engine data revealed that when the start of injection (SOI) was retarded to very late timings, combustion luminosity decreased while exhaust NOx emissions increased, causing a “NOx bump.” This data suggested that changes in radiative heat transfer from soot may affect in-cylinder temperatures and subsequent NOx formation. In this study, soot thermometry measurements of in-cylinder temperature and radiative heat transfer were correlated with exhaust NOx to quantify the role of radiative heat transfer on in-cylinder temperatures and NOx formation. The engine was operated at low-load conditions, for which the premixed burn was a significant fraction of the total heat release.

Our previous work applied LIF measurements of in-cylinder fuel distribution to predict CO2, CO, and HC emissions from an HCCI engine under low-load stratified-charge conditions. The prediction method is based on the premise that local fuel-air packets at a given equivalence ratio (characterized using LIF imaging) burn as if in a homogeneous charge at the same equivalence ratio. Thus, emissions measured during homogeneous operation provide an emission-versus- equivalence-ratio look-up table for predicting stratified-charge emissions. The present paper extends the technique to predict engine-out NOX emissions. Because of operating-range limitations, NOX look-up data for homogeneous operation cannot adequately be determined by experiment. Instead, a CHEMKIN-based model provides this look-up table data instead.

Low-temperature gasoline combustion (LTGC) engines can provide high efficiencies and extremely low NOx and particulate emissions, but controlling the combustion timing remains a challenge. This paper explores the potential of Partial Fuel Stratification (PFS) to provide fast control of CA50 in an LTGC engine. Two different compression ratios are used (CR=16:1 and 14:1) that provide high efficiencies and are compatible with mixed-mode SI-LTGC engines. The fuel used is a research grade E10 gasoline (RON 92, MON 85) representative of a regular-grade market gasoline found in the United States. The fuel was supplied with a gasoline-type direct injector (GDI) mounted centrally in the cylinder. To create the PFS, the GDI injector was pulsed twice each engine cycle. First, an injection early in the intake stroke delivered the majority of the fuel (70 - 80%), establishing the minimum equivalence ratio in the charge.

The impact of 50 ppm intake seeding of ozone (O3) on performance and emissions characteristics was explored in a single-cylinder research engine operated under lean spark assisted compression ignition (SACI) conditions. Optical access into the engine enabled complementary crank angle resolved measurements of in-cylinder O3 concentration via ultraviolet (UV) light absorption. Experiments were performed at moderate loads (4 - 5 bar indicated mean effective pressure) and low-to-moderate engine speeds (800 - 1400 revolutions per minute). Each operating condition featured a single early main injection and maximum brake torque spark timing. Intake pressure was fixed at 1.0 bar, while intake temperatures were varied between 42 - 80 °C. Moderate amounts of internal residuals (12 - 20%) were retained through the use of positive valve overlap. Ozone addition was to found stabilize combustion relative to similar conditions without O3 addition by promoting end gas auto-ignition.

Compliance with future ultra-low nitrogen oxide regulations with diesel engines requires the fastest possible heating of the exhaust aftertreatment system to its proper operating temperature upon cold starting. Late post injections are commonly integrated into catalyst-heating operating strategies. This experimental study provides insight into the complex interactions between the injection-strategy calibration and the tradeoffs between exhaust heat and pollutant emissions. Experiments are performed with certification diesel fuel and blends of diesel fuel with butylal and hexyl hexanoate. Further analyses of experimental data provide insight into fuel reactivity and oxygen content as potential enablers for improved catalyst-heating operation. A statistical design-of-experiments approach is developed to investigate a wide range of injection strategy calibrations at three different intake dilution levels.

The influence of early induction stroke direct injection on late-cycle flows was investigated for a lean-burn, high-tumble, gasoline engine. The engine features side-mounted injection and was operated at a moderate load (8.5 bar brake mean effective pressure) and engine speed (2000 revolutions per minute) condition representative of a significant portion of the duty cycle for a hybridized powertrain system. Thermodynamic engine tests were used to evaluate cam phasing, injection schedule, and ignition timing such that an optimal balance of acceptable fuel economy, combustion stability, and engine-out nitrogen oxide (NOx) emissions was achieved. A single cylinder of the 4-cylinder thermodynamic engine was outfitted with an endoscope that enabled direct imaging of the spark discharge and early flame development.

Previous work has shown that conventional diesel ignition improvers, 2-ethylhexyl nitrate (EHN) and di-tert-butyl peroxide (DTBP), can be used to enhance the autoignition of a regular-grade E10 gasoline in a well premixed low-temperature gasoline combustion (LTGC) engine, hereafter termed an HCCI engine, at naturally aspirated and moderately boosted conditions (up to 180 kPa absolute) with a constant engine speed of 1200 rpm and a 14:1 compression ratio. In the current work the effect of EHN on boosted HCCI combustion is further investigated with a higher compression ratio (16:1) piston and over a range of engine speeds (up to 2400 rpm). The results show that the higher compression ratio and engine speeds can make the combustion of a regular-grade E10 gasoline somewhat less stable. The addition of EHN improves the combustion stability by allowing combustion phasing to be more advanced for the same ringing intensity.

Nitric Oxide (NO) can significantly influence the autoignition reactivity and this can affect knock limits in conventional stoichiometric SI engines. Previous studies also revealed that the role of NO changes with fuel type. Fuels with high RON (Research Octane Number) and high Octane Sensitivity (S = RON - MON (Motor Octane Number)) exhibited monotonically retarding knock-limited combustion phasing (KL-CA50) with increasing NO. In contrast, for a high-RON, low-S fuel, the addition of NO initially resulted in a strongly retarded KL-CA50 but beyond the certain amount of NO, KL-CA50 advanced again. The current study focuses on same high-RON, low-S Alkylate fuel to better understand the mechanisms responsible for the reversal in the effect of NO on KL-CA50 beyond a certain amount of NO.

Methanol is one of the most promising fuels for the decarbonization of the off-road and transportation sectors. Although methanol is typically seen as an alternative fuel for spark ignition engines, mixing-controlled compression ignition (MCCI) combustion is typically preferred in most off-road and medium-and heavy-duty applications due to its high reliability, durability and high-efficiency. In this paper, the potential of using ignition enhancers to enable methanol MCCI combustion was investigated. Methanol was blended with 2-ethylhexyl nitrate (EHN) and experiments were performed in a single-cylinder production-like diesel research engine, which has a displacement volume of 0.83 L and compression ratio of 16:1. The effect of EHN has been evaluated with three different levels (3%vol, 5%vol, and 7%vol) under low- and part-load conditions. The injection timing has been swept to find the stable injection window for each EHN level and load.