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Soot formation process was examined by high speed photographs, using a single cumbustion diesel engine with a transparent swirl chamber. Fuel-air mixture and flames, and soot clouds were visualized by the schlieren method and the back-illuminated method, respectively. A three dimensional simulation program with soot formation and oxidation models was developed to clarify diesel soot formation processes. The models consist of several models previously proposed and partly improved in this study. Good agreement was obtained between calculated and experimental results. The following points were clarified through observation and numerical studies: (1) The main soot area is considerably smaller than luminous flame area, especially in the initial soot formation process. (2) The main soot cloud first appears in the tip region of fuel-air mixture, downstream of ignition position a few submilliseconds after the ignition.

In order to optimize air-fuel mixture formation in a small DI diesel engine, studies were conducted into the effects of combustion chamber shape and fuel spray impingement. Based on the findings of these studies, the shape of the combustion chamber was modified to induce complex air motion with high turbulence and fuel injection was carefully controlled to achieve optimum impingement intensity. As a result, the mixture formation process was greatly improved with a consequent gain in terms of engine performance. To clarify the reasons for this improvement in combustion, a three-dimensional calculation of the in-cylinder air motion was made. The behaviour of the spray and flame was observed using an endoscope. The new combustion system, named TOYOTA Reflex Burn system (TRB) thus developed has been adopted in production engines since August 1988.

This paper deals with oxygen storage effect and NOx conversion reaction modeling. It was found that the oxygen stored in the catalyst increases with catalytic wall temperature and lean ( or rich ) depth from experiments using a well controlled flow reactor. Oxygen storage-release model (OSR model), incorporated with the NOx reduction reaction and THC or CO oxidation reaction, was established from the experimental results. Reaction rate parameters for three-way catalyst have been determined from the least data of flow reactor experiments using Evolutionary Algorithm. Transient temperatures and emissions are predicted using the developed OSR model and the determined reaction rate parameters for three-way catalyst, which are incorporated in the numerical algorithms used in the previous paper to predict flow and temperature field in a catalytic converter.

A three-dimensional numerical model has been developed to predict spray formation process of swirl or slit type injectors which are currently used in direct-injection gasoline engines. The Discrete Droplet Model (DDM) is totally enhanced: a new droplet deformation model is developed, which is theoretically introduced with a spheroidal shape assumption. The droplet drag model and droplet break-up model via Kelvin-Helmholtz and Rayleigh-Taylor instabilities are modified taken into account with the deformation. The break-up model parameters are dynamically changed according to a droplet Weber number. The model functions are developed using single droplet breakup measurement data. A liquid sheet injection and breakup models are incorporated into the DDM. A new parcel radius model is also introduced to get rid of the grid dependence of the droplet collision-coalescence model.

Methanol steam reforming, which is an endothermic reaction, needs some heating. Both methanol conversion ratio and carbon monoxide (CO) concentration increase when temperature is elevated. As CO poisons a typical polymer electrolyte of a fuel cell, the relationship between methanol conversion ratio and CO concentration is a trade-off one. It was found from preliminary researches that the reforming reaction speed is controlled by heat transfer rate at large methanol flow rate, where methanol conversion ratio becomes lower and CO concentration becomes higher. Therefore it is necessary to develop a new methanol reforming concept that provides stable combustion for heating and enhanced heat transfer for improving the trade-off relationship and making a compact reformer. Reforming catalyst using metal honeycomb support and a new catalytic combustion were applied to a new concept plate type methanol steam reformer, which is used in a fuel cell of 3 kW-class electric generation.

In direct-injection (DI) gasoline engines, spray characteristics greatly affect engine combustion. For the rapid development of new gasoline direct-injectors, it is necessary to predict the spray characteristics accurately by numerical analysis based on the injector nozzle geometry. In this study, two-phase flow inside slit nozzle injectors is calculated using the volume of fluid method in a three-dimensional CFD. The calculation results are directly applied to the boundary conditions of spray calculations, of which the submodels are recently developed to predict spray formation process in direct injection gasoline engines. The calculation results are compared with the experiments. Good agreements are obtained for typical spray characteristics such as spray shape, penetration and Sauter mean diameter at both low and high ambient pressures. Two slit nozzle injectors of which the slit thickness is different are compared.

It was shown in our previous study that the air-jet in the late combustion period reduces the diesel exhaust soot effectively. However, the plunger-pump type air-jet generator used in our previous study has a big power-loss. In this paper, the reduction of soot emission with a newly designed air-accumulation type air-jet generator is investigated using an experimental single cylinder engine. The optimum design parameters, such as the spring constant and the air outlet diameter, are examined experimentally. The effectiveness of the air-accumulation type air-jet generator for the reduction of soot and NOx emission is about a half of that of the plunger-pump type. It is confirmed that the disappearing speed of the luminous flame region accelerates with the increase of the heat-release in the late combustion period.

A new spray/wall impingement model for gasoline engines has been developed. The model is based on experimental analysis of impinging spray droplets using a phase doppler particle analizer (PDPA). Three new equations were obtained in terms of droplet size, Weber number and the angle from a wall for droplets which were splashed after impinging or created by the impact of a droplet on the liquid film layer on the wall. The three-dimensional calculation results using the model agree very well with the experimental data. The model is also applied to the fuel mixture formation process in a lean-burn gasoline engine.

Transient temperature and concentration distribution inside a catalytic converter during warm-up have been analyzed by experiments and numerical simulation. There is great maldistribution of species concentrations inside a converter during warm-up. Carbon monoxide (CO) and hydrocarbons (HC) have high concentrations in the exhaust gas passing through outer region cells because they are not converted due to low wall temperature. The effects of the noble metal loading pattern on conversion characteristics during warm-up have been investigated by numerical simulation. The effects of high-loading on improving conversion characteristics are saturated with the loading quantity of six times that of the base-loading. High-loading of the noble metal only on the frontal region (20 or 30mm. from the front face) has almost the same warming-up conversion performance as the uniform high-loading.

Three-dimensional numerical analysis of fuel liquid and mixture behavior in a port-injection gasoline engine is assessed by comparing calculations with measurements. The fuel mass distributed in the intake port and cylinder is measured using an engine with hydraulic valve and gas sampling system. The experimental results show that about half of the fuel mass per injection enters the cylinder, and the rest stays in the port. The difference of the mass fraction of injected fuel directly entering the cylinder is small between the cases of single pulse injection and serial injection. Therefore, three-dimensional calculation presupposing single pulse injection has difficulty in predicting the in-cylinder mixture formation process, although it can analyze the amount of fuel wetting the port wall. The calculations are performed for a port-injection engine, and the differences of fuel behavior with respect to swirl control valve opening and wall temperature are discussed.

A series calculation methodology from the injector nozzle internal flow to the in-cylinder fuel spray and mixture formation in a diesel engine was developed. The present method was applied to a valve covered orifice (VCO) nozzle with the recent common rail injector system. The nozzle internal flow calculation using an Eulerian three-fluid model and a cavitation model was performed. The needle valve movement during the injection period was taken into account in this calculation. Inside the nozzle hole, cavitation appears at the nozzle hole inlet edge, and the cavitation region separates into two regions due to a secondary flow in the cross section, and it is distributed to the nozzle exit. Unsteady change of the secondary flow caused by needle movement affects the cavitation distribution in the nozzle hole, and the spread angle of the velocity vector at the nozzle exit.

A new type closed loop A/F control carburetor has been developed. In the carburetor, an air jet, a by-pass stream of an intake air flow, is made to collide with a fuel flow to suppress the flow rate. Studies were made of the basic features of the method such as fuel controlling capability and the factors affecting it from phenomenological consideration and schlieren observation. For comparison, three types of carburetors were prepared for the conbination of main and idle fuel circuits. In driving mode tests on a dynamometer, a new carburetor which employs the new method for the main fuel circuit, provides 30 % lower emission level than an air bleed control carburetor. Higher controlling frequencies were obtained for the new carburetors. The high controllability of the air jet collision control method is attributable to the smaller fluctuation in both the controlling air and the spouting fuel.

This paper presents the numerical simulation method to predict the deactivation process of three-way catalytic converters. Three-way catalytic converter's deactivation typically results from thermal and chemical mechanisms. The major factor of thermal deactivation is the sintering of noble metal particles, which is known to depend on the ageing temperature and the oxygen concentration in the exhaust gas. The chemical deactivation is mainly caused by the poisoning, which has two effects on the catalyst deactivation. One effect is the loss of the catalyst activity, which is expressed by reduced frequency factors of reaction rates. Another effect is the suppression of the noble metal sintering. Poison deposits prevent the noble metal particles from moving in the washcoat, assisted by the reduced thermal loading of reaction heats, which is caused by the loss of the catalyst activity. Modeling these deactivation factors, we propose the rate expression of noble metal sintering.

A multi-component fuel vaporization model is developed for numerical analysis of specific fuel component behaviors in port-fuel-injection(PFI) gasoline engines. In order to specify the differences of in-cylinder fuel distribution among its components, three-dimensional calculations of intake flow, spray and vapor motion of each component are performed with respect to engine wall temperature and the distillation characteristics of the fuel. Simultaneous measurements of in-cylinder behaviors of different volatility components in the fuel are also carried out using a laser-induced fluorescence (LIF) technique to validate the calculation results. In both measurements and calculations, the same fuels are used, which are composed of seven or eight components to simulate the distillation characteristics of two kinds of gasoline. The in-cylinder vapor amount of high and low volatility components is compared between the calculations and the experiments.

This report describes the implementation of the spark channel short circuit and blow-out submodels, which were described in the previous report, into a spark ignition model. The spark channel which is modeled by a particle series is elongated by moving individual spark particles along local gas flows. The equation of the spark channel resistance developed by Kim et al. is modified in order to describe the behavior of the current and the voltage in high flow velocity conditions and implemented into the electrical circuit model of the electrical inductive system of the spark plug. Input parameters of the circuit model are the following: initial discharge energy, inductance, internal resistance and capacitance of the spark plug, and the spark channel length obtained by the spark channel model. The instantaneous discharge current and the voltage are obtained as outputs of the circuit model.

The spray characteristics and inside flow of a marine diesel injector were investigated both experimentally and numerically. From the experiments, we observed that the penetration of the sprays in the early injection stage gradually increases. This phenomenon differs significantly from that of the small automobile diesel injector, in which penetration increases linearly with time. Using the momentum method to obtain injection rate measurements, we observed an injection rate spike at each injection event just after the injection began. The observed spray results show that the small portion of fuel remaining inside the nozzle from the previous injection event is ejected first, and then the main volume of fuel is ejected. Both fuels accumulate as spray droplets and gradually accelerate after the early injection stage. Numerical simulations of the injector's inside flow show that the fuel injection rate becomes saturated in needle lifts larger than 0.3 mm.

For the measurements of flow rate, pressure and/or temperature in an engine exhaust pipe, probes are often inserted into the exhaust pipe depending on the application. These measurement probes differ a lot in terms of their size and shape. The flow around the probes become further complicated due to the pulsation of engine exhaust flow. In this study, computational fluid dynamics (CFD) simulations were carried out and a zero-dimensional (0D) model was constructed to analyze the flow field around the probe and flow rate of a pulsating flow. The simulations and the measurements of the flow rate and pressure were performed on flows around a hexagonal prism inserted in a circular pipe which is intended to be a differential pressure flow meter. The velocity field was also measured using the particle image velocimetry (PIV) technique. The CFD simulation results were validated with the experiments for both steady and pulsating flows.