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To achieve an accurate estimate of losses in a battery it is necessary to consider the reversible entropic losses, which may constitute over 20% of the peak total loss. In this work, a procedure for experimentally determining the entropic heating coefficient of a lithium-ion battery cell is developed. The entropic heating coefficient is the rate of change of the cell’s open-circuit voltage (OCV) with respect to temperature; it is a function of state-of-charge (SOC) and temperature and is often expressed in mV/K. The reversible losses inside the cell are a function of the current, the temperature, and the entropic heating coefficient, which itself is dependent on the cell chemistry. The total cell losses are the sum of the reversible and irreversible losses, where the irreversible losses consist of ohmic losses in the electrodes, ion transport losses, and other irreversible chemical reactions.

A large amount of heat is generated in electric vehicle battery packs during high rate charging, resulting in the need for effective cooling methods. In this paper, a prototype liquid cooled large format Lithium-ion battery module is modeled and tested. Experiments are conducted on the module, which includes 31Ah NMC/Graphite pouch battery cells sandwiched by a foam thermal pad and heat sinks on both sides. The module is instrumented with twenty T-type thermocouples to measure thermal characteristics including the cell and foam surface temperature, heat flux distribution, and the heat generation from batteries under up to 5C rate ultra-fast charging. Constant power loss tests are also performed in which battery loss can be directly measured.